Carbon Dioxide Efficiency of Terrestrial Enhanced Weathering
Abstract
Terrestrial enhanced weathering, the spreading of ultramafic silicate rock flour to enhance natural weathering rates, has been suggested as part of a strategy to reduce global atmospheric CO2 levels. We budget potential CO2 sequestration against associated CO2 emissions to assess the net CO2 removal of terrestrial enhanced weathering. We combine global spatial data sets of potential source rocks, transport networks, and application areas with associated CO2 emissions in optimistic and pessimistic scenarios. The results show that the choice of source rocks and material comminution technique dominate the CO2 efficiency of enhanced weathering. CO2 emissions from transport amount to on average 0.5-3% of potentially sequestered CO2. The emissions of material mining and application are negligible. After accounting for all emissions, 0.5-1.0 t CO2 can be sequestered on average per tonne of rock, translating into a unit cost from 1.6 to 9.9 GJ per tonne CO2 sequestered by enhanced weathering. However, to control or reduce atmospheric CO2 concentrations substantially with enhanced weathering would require very large amounts of rock. Before enhanced weathering could be applied on large scales, more research is needed to assess weathering rates, potential side effects, social acceptability, and mechanisms of governance.
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Integrity signals
Registry
Cites
Statistics
Claims the paper makes
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Claims other papers make about this one
Each is checked against this paper’s own text: does it say what the citing paper says it does?
Rock grinding to reduce particle size and maximise CDR is the primary energy consuming operation in ERW.
“Rock grinding to reduce particle size and maximise CDR is the primary energy consuming operation in ERW 22,23,73 .”
From Potential for large-scale CO2 removal via enhanced rock weathering with croplands (2020) · cites this paper as [73]
Our approach improves on prior analyses that assumed a fixed radius between rock dust source and site of application.
“Our approach improves on prior analyses, which assumed a fixed radius between rock dust source and site of application 73 .”
From Potential for large-scale CO2 removal via enhanced rock weathering with croplands (2020) · cites this paper as [73]
Self-check
Percentages, sums and reported differences re-computed from the paper’s own numbers.
The self-check needs the paper’s full text.
Cites
World map of the Köppen-Geiger climate classification updated
Kottek, M., Grieser, J., Beck, C., Rudolf, B., & Rubel, F. (2006) · Meteorologische Zeitschrift · doi:10.1127/0941-2948/2006/0130 · Cited by 11,456 · see citing works
A global map of human impact on marine ecosystems
Halpern, B. S., Walbridge, S., Selkoe, K. A., Kappel, C. V., Micheli, F., D'Agrosa, C., Bruno, J. F., Casey, K. S., Ebert, C., Fox, H. E., et al. (2008) · Science · doi:10.1126/science.1149345 · Cited by 6,627 · see citing works
The story of phosphorus: Global food security and food for thought
Cordell, D., Drangert, J.-O., & White, S. B. (2009) · Global Environmental Change · doi:10.1016/j.gloenvcha.2008.10.009 · Cited by 5,243 · see citing works
Global silicate weathering and CO2 consumption rates deduced from the chemistry of large rivers
Gaillardet, J., Dupré, B., Louvat, P., & Allègre, C. J. (1999) · Chemical Geology · doi:10.1016/s0009-2541(99)00031-5 · Cited by 3,334 · see citing works
Berner, R. A., Lasaga, A. C., & Garrels, R. M. (1983) · American Journal of Science · doi:10.2475/ajs.283.7.641 · Cited by 2,428 · see citing works
A negative feedback mechanism for the long‐term stabilization of Earth's surface temperature
Walker, J. C. G., Hays, P. B., & Kasting, J. F. (1981) · Journal of Geophysical Research: Oceans · doi:10.1029/jc086ic10p09776 · Cited by 2,310 · see citing works
The anomaly of silicon in plant biology.
Epstein, E. Z. (1994) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.91.1.11 · Cited by 1,740 · see citing works
Global chemical weathering of surficial rocks estimated from river dissolved loads
Meybeck, M. (1987) · American Journal of Science · doi:10.2475/ajs.287.5.401 · Cited by 1,633 · see citing works
Hartmann, J., & Moosdorf, N. (2012) · Geochemistry Geophysics Geosystems · doi:10.1029/2012gc004370 · Cited by 1,168 · see citing works
Self-citationHeavy metals in soils: trace metals and metalloids in soils and their bioavailability
(2013) · Choice Reviews Online · doi:10.5860/choice.50-3862 · Cited by 1,067 · see citing works
Basalt weathering laws and the impact of basalt weathering on the global carbon cycle
Dessert, C., Dupré, B., Gaillardet, J., François, L., & Allègre, C. J. (2003) · Chemical Geology · doi:10.1016/j.chemgeo.2002.10.001 · Cited by 998 · see citing works
CO2 disposal by means of silicates
SEIFRITZ, W. (1990) · Nature · doi:10.1038/345486b0 · Cited by 956 · see citing works
Rapid growth in CO2 emissions after the 2008–2009 global financial crisis
Peters, G. P., Marland, G., Quéré, C. L., Boden, T. A., Canadell, J. G., & Raupach, M. (2011) · Nature Climate Change · doi:10.1038/nclimate1332 · Cited by 871 · see citing works
In situ carbonation of peridotite for CO <sub>2</sub> storage
Kelemen, P. B., & Matter, J. (2008) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0805794105 · Cited by 750 · see citing works
Hartmann, J., West, A. J., Renforth, P., Köhler, P., De La Rocha, C. L., Wolf‐Gladrow, D. A., Dürr, H. H., & Scheffran, J. (2013) · Reviews of Geophysics · doi:10.1002/rog.20004 · Cited by 717 · see citing works
Self-citationGorbushina, A. A. (2007) · Environmental Microbiology · doi:10.1111/j.1462-2920.2007.01301.x · Cited by 640 · see citing works
Ex situ aqueous mineral carbonation
Gerdemann, S. J., O'Connor, W. K., Dahlin, D. C., Penner, L. R., & Rush, H. (2007) · Environmental Science & Technology · doi:10.1021/es0619253 · Cited by 633 · see citing works
Amiotte Suchet, P., Probst, J., & Ludwig, W. (2003) · Global Biogeochemical Cycles · doi:10.1029/2002gb001891 · Cited by 606 · see citing works
Riebe, C. S., Kirchner, J. W., & Finkel, R. C. (2004) · Earth and Planetary Science Letters · doi:10.1016/j.epsl.2004.05.019 · Cited by 585 · see citing works
Enhanced Weathering: An Effective and Cheap Tool to Sequester Co2
Schuiling, R. D., & Krijgsman, P. (2006) · Climatic Change · doi:10.1007/s10584-005-3485-y · Cited by 403 · see citing works
Geoengineering potential of artificially enhanced silicate weathering of olivine
Köhler, P., Hartmann, J., & Wolf-Gladrow, D. A. (2010) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1000545107 · Cited by 384 · see citing works
Self-citationHartmann, J., Jansen, N., Dürr, H. H., Kempe, S., & Köhler, P. (2009) · Global and Planetary Change · doi:10.1016/j.gloplacha.2009.07.007 · Cited by 382 · see citing works
Self-citationHartmann, J., Moosdorf, N., Lauerwald, R., Hinderer, M., & West, A. J. (2013) · Chemical Geology · doi:10.1016/j.chemgeo.2013.10.025 · Cited by 355 · see citing works
Self-citationThe Role of Fungi in Weathering
Hoffland, E., Kuyper, T. W., Wallander, H., Plassard, C., Gorbushina, A. A., Haselwandter, K., Holmström, S., Landeweert, R., Lundström, U. S., Rosling, A., et al. (2004) · Frontiers in Ecology and the Environment · doi:10.1890/1540-9295(2004)002[0258:trofiw]2.0.co;2 · Cited by 341 · see citing works
Moulton, K. L. (2000) · American Journal of Science · doi:10.2475/ajs.300.7.539 · Cited by 308 · see citing works
GlobCover: ESA service for global land cover from MERIS
Arino, O., Gross, D., Ranera, F., Leroy, M., Bicheron, P., Brockman, C., Defourny, P., Vancutsem, C., Achard, F., Durieux, L., et al. (2007) · 2007 IEEE International Geoscience and Remote Sensing Symposium · doi:10.1109/igarss.2007.4423328 · Cited by 302 · see citing works
A review of climate geoengineering proposals
Vaughan, N. E., & Lenton, T. M. (2011) · Climatic Change · doi:10.1007/s10584-011-0027-7 · Cited by 297 · see citing works
Mineral stimulation of subsurface microorganisms: release of limiting nutrients from silicates
Rogers, J. R., & Bennett, P. C. (2003) · Chemical Geology · doi:10.1016/j.chemgeo.2003.09.001 · Cited by 296 · see citing works
Caldeira, K., Bala, G., & Cao, L. (2013) · Annual Review of Earth and Planetary Sciences · doi:10.1146/annurev-earth-042711-105548 · Cited by 270 · see citing works
The potential of enhanced weathering in the UK
Renforth, P. (2012) · International journal of greenhouse gas control · doi:10.1016/j.ijggc.2012.06.011 · Cited by 265 · see citing works
Self-citationBrady, P. V., & Carroll, S. A. (1994) · Geochimica et Cosmochimica Acta · doi:10.1016/0016-7037(94)90543-6 · Cited by 253 · see citing works
Gadikota, G., Matter, J., Kelemen, P., & Park, A.-H. A. (2014) · Physical Chemistry Chemical Physics · doi:10.1039/c3cp54903h · Cited by 247 · see citing works
A comparative global assessment of potential negative emissions technologies
McLaren, D. P. (2012) · Process Safety and Environmental Protection · doi:10.1016/j.psep.2012.10.005 · Cited by 245 · see citing works
Farming with rocks and minerals: challenges and opportunities
van Straaten, P. (2006) · Anais da Academia Brasileira de Ciências · doi:10.1590/s0001-37652006000400009 · Cited by 232 · see citing works
Hangx, S. J. T., & Spiers, C. J. (2009) · International journal of greenhouse gas control · doi:10.1016/j.ijggc.2009.07.001 · Cited by 228 · see citing works
CO2 efficiency in road freight transportation: Status quo, measures and potential
Léonardi, J., & Baumgartner, M. (2004) · Transportation Research Part D Transport and Environment · doi:10.1016/j.trd.2004.08.004 · Cited by 222 · see citing works
Hanghøj, K., Kelemen, P. B., Hassler, D., & Godard, M. (2010) · Journal of Petrology · doi:10.1093/petrology/egp077 · Cited by 195 · see citing works
Herbivore specific induction of silica-based plant defences
Massey, F. P., Ennos, A. R., & Hartley, S. E. (2007) · Oecologia · doi:10.1007/s00442-007-0703-5 · Cited by 191 · see citing works
Effect of Calcium Silicate on Blast and Brown Spot Intensities and Yields of Rice
Datnoff, L. E. (1991) · Plant Disease · doi:10.1094/pd-75-0729 · Cited by 184 · see citing works
Measurement of CO2 emissions from road freight transport: A review of UK experience
McKinnon, A. C., & Piecyk, M. I. (2009) · Energy Policy · doi:10.1016/j.enpol.2009.07.007 · Cited by 173 · see citing works
ten Berge, H. F. M., van der Meer, H. G., Steenhuizen, J. W., Goedhart, P. W., Knops, P. C. M., & Verhagen, A. (2012) · PLoS ONE · doi:10.1371/journal.pone.0042098 · Cited by 172 · see citing works
Industrial and Process Furnaces: Principles, Design and Operation
Mullinger, P. J., & Jenkins, B. (2008) · doi:10.1016/c2012-0-02745-7 · Cited by 121 · see citing works
Schopka, H. H., Derry, L. A., & Arcilla, C. A. (2010) · Geochimica et Cosmochimica Acta · doi:10.1016/j.gca.2010.11.014 · Cited by 116 · see citing works
Engineering challenges of ocean liming
Renforth, P., Jenkins, B., & Kruger, T. (2013) · Energy · doi:10.1016/j.energy.2013.08.006 · Cited by 112 · see citing works
Self-citationManning, D. A. C., Renforth, P., Lopez-Capel, E., Robertson, S., & Ghazireh, N. (2013) · International journal of greenhouse gas control · doi:10.1016/j.ijggc.2013.05.012 · Cited by 106 · see citing works
Rozalen, M., Huertas, F. J., & Brady, P. R. (2009) · Geochimica et Cosmochimica Acta · doi:10.1016/j.gca.2009.03.026 · Cited by 100 · see citing works
Leake, J. R., Duran, A. L., Hardy, K., et al. (2008) · Mineralogical Magazine · doi:10.1180/minmag.2008.072.1.85 · Cited by 99 · see citing works
Passive Sequestration of Atmospheric CO2 through Coupled Plant-Mineral Reactions in Urban soils
Manning, D. A. C., & Renforth, P. (2012) · Environmental Science & Technology · doi:10.1021/es301250j · Cited by 89 · see citing works
Self-citationImpact of alkalinity sources on the life-cycle energy efficiency of mineral carbonation technologies
Kirchofer, A., Brandt, A., Krevor, S., Prigiobbe, V., & Wilcox, J. (2012) · Energy & Environmental Science · doi:10.1039/c2ee22180b · Cited by 81 · see citing works
Atmospheric CO2 consumption by chemical weathering in North America
Moosdorf, N., Hartmann, J., Lauerwald, R., Hagedorn, B., & Kempe, S. (2011) · Geochimica et Cosmochimica Acta · doi:10.1016/j.gca.2011.10.007 · Cited by 79 · see citing works
Self-citationMeasuring and Managing CO2 Emissions of European Chemical Transport
McKinnon, A. C., & Piecyk, M. I. (2011) · Zenodo (CERN European Organization for Nuclear Research) · doi:10.5281/zenodo.10783090 · Cited by 75 · see citing works
Structural changes in olivine (Mg, Fe)2SiO4 mechanically activated in high-energy mills
Baláž, P., Turianicová, E., Fabián, M., Kleiv, R. A., Briančin, J., & Obut, A. (2008) · International Journal of Mineral Processing · doi:10.1016/j.minpro.2008.04.001 · Cited by 72 · see citing works
Chizmeshya, A. V. G., McKelvy, M. J., Squires, K., et al. (2007) · doi:10.2172/924162 · Cited by 28 · see citing works
Flagged first, then by citations
Research works printed but not linked: 4
- [12]12. Kempe, S., Carbon in the rock cycle. In The Global Carbon Cycle , Bolin, B.; Degens, E. 379 380 T.; Kempe, S.; Ketner, P., Eds. Scientific Committee On Problems of the Environment (SCOPE): - Old Woking, 1979; Vol. 13, pp 343-375. 381
- [43]43. Kelemen, P. B.; Matter, J., In situ carbonation of peridotite for CO2 storage. Proceedings 463 464 of the National Academy of Sciences of the United States of America 17300. 465
- [3]3. edition, 1:5,000,000 In Commission for the Geological World Map: 2010. 467
- [6]6. Element Geochemistry, and Os Isotope and PGE Systematics. Journal of Petrology 2010, 51 , (1470
Cited by
Sorted by citations
Potential for large-scale CO2 removal via enhanced rock weathering with croplands
Beerling, D. J., Kantzas, E. P., Lomas, M. R., Wade, P., Eufrasio, R. M., Renforth, P., Sarkar, B., Andrews, M. G., James, R. H., Pearce, C. R., et al. (2020) · Nature · doi:10.1038/s41586-020-2448-9 · Cited by 700 · see citing works
Self-citationAssessing ocean alkalinity for carbon sequestration
Renforth, P., & Henderson, G. (2017) · Reviews of Geophysics · doi:10.1002/2016rg000533 · Cited by 655 · see citing works
Self-citationFarming with crops and rocks to address global climate, food and soil security
Beerling, D. J., Leake, J. R., Long, S. P., Scholes, J. D., Ton, J., Nelson, P. N., Bird, M., Kantzas, E., Taylor, L. L., Sarkar, B., et al. (2018) · Nature Plants · doi:10.1038/s41477-018-0108-y · Cited by 480 · see citing works
Smith, P., Adams, J., Beerling, D. J., Beringer, T., Calvin, K. V., Fuss, S., Griscom, B., Hagemann, N., Kammann, C., Kraxner, F., et al. (2019) · Annual Review of Environment and Resources · doi:10.1146/annurev-environ-101718-033129 · Cited by 380 · see citing works
Self-citationPotential and costs of carbon dioxide removal by enhanced weathering of rocks
Strefler, J., Amann, T., Bauer, N., Kriegler, E., & Hartmann, J. (2018) · Environmental Research Letters · doi:10.1088/1748-9326/aaa9c4 · Cited by 372 · see citing works
Self-citationEnhanced weathering strategies for stabilizing climate and averting ocean acidification
Taylor, L. L., Quirk, J., Thorley, R. M. S., Kharecha, P. A., Hansen, J., Ridgwell, A., Lomas, M. R., Banwart, S. A., & Beerling, D. J. (2016) · Nature Climate Change · doi:10.1038/nclimate2882 · Cited by 366 · see citing works
Negative emissions—Part 3: Innovation and upscaling
Nemet, G. F., Callaghan, M. W., Creutzig, F., Fuss, S., Hartmann, J., Hilaire, J., Lamb, W. F., Minx, J. C., Rogers, S., & Smith, P. (2018) · Environmental Research Letters · doi:10.1088/1748-9326/aabff4 · Cited by 343 · see citing works
Self-citationOlivine dissolution rates: A critical review
Oelkers, E. H., Declercq, J., Saldi, G. D., Gislason, S. R., & Schott, J. (2018) · Chemical Geology · doi:10.1016/j.chemgeo.2018.10.008 · Cited by 296 · see citing works
Kelland, M. E., Wade, P. W., Lewis, A. L., Taylor, L. L., Sarkar, B., Andrews, M. G., Lomas, M. R., Cotton, T. E. A., Kemp, S. J., James, R. H., et al. (2020) · Global Change Biology · doi:10.1111/gcb.15089 · Cited by 281 · see citing works
Young people's burden: requirement of negative CO <sub>2</sub> emissions
Hansen, J., Sato, M., Kharecha, P., von Schuckmann, K., Beerling, D. J., Cao, J., Marcott, S., Masson-Delmotte, V., Prather, M. J., Rohling, E. J., et al. (2017) · Earth System Dynamics · doi:10.5194/esd-8-577-2017 · Cited by 266 · see citing works
Potential CO2 removal from enhanced weathering by ecosystem responses to powdered rock
Goll, D. S., Ciais, P., Amann, T., Buermann, W., Chang, J., Eker, S., Hartmann, J., Janssens, I., Li, W., Obersteiner, M., et al. (2021) · Nature Geoscience · doi:10.1038/s41561-021-00798-x · Cited by 197 · see citing works
Self-citationPyrogenic carbon capture and storage
Schmidt, H., Anca‐Couce, A., Hagemann, N., Werner, C., Gerten, D., Lucht, W., & Kammann, C. (2019) · GCB Bioenergy · doi:10.1111/gcbb.12553 · Cited by 186 · see citing works
Lefebvre, D., Goglio, P., Williams, A., Manning, D. A. C., de Azevedo, A. C., Bergmann, M., Meersmans, J., & Smith, P. (2019) · Journal of Cleaner Production · doi:10.1016/j.jclepro.2019.06.099 · Cited by 153 · see citing works
Fossil fuels in a trillion tonne world
Scott, V., Haszeldine, R. S., Tett, S. F. B., & Oschlies, A. (2015) · Nature Climate Change · doi:10.1038/nclimate2578 · Cited by 124 · see citing works
Power, I. M., Dipple, G. M., Bradshaw, P. M. D., & Harrison, A. L. (2020) · International Journal of Greenhouse Gas Control · doi:10.1016/j.ijggc.2019.102895 · Cited by 84 · see citing works
Ideas and perspectives: Synergies from co-deployment of negative emission technologies
Amann, T., & Hartmann, J. (2019) · Biogeosciences · doi:10.5194/bg-16-2949-2019 · Cited by 53 · see citing works
Self-citationReview and outlook for agromineral research in agriculture and climate mitigation
Zhang, G., Kang, J., Wang, T., & Zhu, C. (2018) · Soil Research · doi:10.1071/sr17157 · Cited by 32 · see citing works
- Authors
- Moosdorf, N., Renforth, P., & Hartmann, J.
- Affiliations
- Universität Hamburg (DE)
- University of Oxford (GB)
- Corresponding author
- Moosdorf, Nils
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-04-08
- Volume
- 48
- Issue
- 9
- Pages
- 4809-4816
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2018921467
- Cited by
- 207
- References
- 53
- Citations by year
- 2026: 23 · 2025: 27 · 2024: 30 · 2023: 36 · 2022: 18 · 2021: 17 · 2020: 9 · 2019: 14 · 2018: 10 · 2017: 10 · 2016: 4 · 2015: 7 · 2014: 2
- FWCI
- 5.88
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Environmental Science & Technology (publishedVersion)
- PubMed (publishedVersion)
- ORCA Online Research @Cardiff (Cardiff University) (acceptedVersion)
- Helmholtz Centre for Ocean Research Kiel (GEOMAR) (acceptedVersion)
- Max Planck Digital Library (submittedVersion)
- ORCA Online Research @Cardiff (Cardiff University) (submittedVersion)
- MPG.PuRe (Max Planck Society) (submittedVersion)
- Topics
- Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
- Physical Sciences › Engineering › Mechanical Engineering › Carbon Dioxide Capture Technologies
- Physical Sciences › Environmental Science › Global and Planetary Change › Climate Change and Geoengineering
- Keywords
- CO2 sequestration, carbon dioxide removal, ultramafic rocks, transport emissions, geoengineering, atmospheric CO2 reduction
- MeSH terms
- Carbon Dioxide, Weather, Silicates
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
Are you an author, or do you see a problem with this page? Request a review