Cited by 314Advanced oxidation water treatmentWater Treatment and DisinfectionAdvanced Photocatalysis Techniques

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Degradation of antipyrine by UV, UV/H2O2 and UV/PS

Tan, Chaoqun, Gao, Naiyun, Deng, Yang, Zhang, Yongji, Sui, Minghao, Deng, Jing, Zhou, Shiqing·2013·Journal of Hazardous Materials

DOI 10.1016/j.jhazmat.2013.06.060

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Abstract

Degradation of antipyrine (AP) in water by three UV-based photolysis processes (i.e., direct UV, UV/H₂O₂, UV/persulfate (UV/PS)) was studied. For all the oxidation processes, the AP decomposition exhibited a pseudo-first-order kinetics pattern. Generally, UV/H₂O₂ and UV/PS significantly improved the degradation rate relevant to UV treatment alone. The pseudo-first-order degradation rate constants (kobs) were, to different degrees, affected by initial AP concentration, oxidant dose, pH, UV irradiation intensity, and co-existing chemicals such as humic acid, chloride, bicarbonate, carbonate and nitrate. The three oxidation processes followed the order in terms of treatment costs: UV/PS>UV>UV/H₂O₂ if the energy and chemical costs are considered. Finally, the AP degradation pathways in the UV/H₂O₂ and UV/PS processes are proposed. Results demonstrated that UV/H₂O₂ and UV/PS are potential alternatives to control water pollution caused by emerging contaminants such as AP.

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Authors: Tan, C., Gao, N., Deng, Y., Zhang, Y., Sui, M., Deng, J., & Zhou, S.
Affiliations: Tongji University (CN)
Corresponding author: Gao, Naiyun
ORCID: Tan, Chaoqun
Gao, Naiyun
Deng, Yang
Zhang, Yongji
Sui, Minghao
Deng, Jing
Zhou, Shiqing
Venue: Journal of Hazardous Materials
Publisher: Elsevier BV
Published: 2013-09
Volume: 260
Pages: 1008-1016
ISSN: 0304-3894 (ISSN-L)
DOI: 10.1016/j.jhazmat.2013.06.060
OpenAlex: W1967091842
Cited by: 314
References: 44
Citations by year: 2026: 10 · 2025: 15 · 2024: 27 · 2023: 27 · 2022: 27 · 2021: 24 · 2020: 35 · 2019: 37 · 2018: 36 · 2017: 19 · 2016: 32 · 2015: 12 · 2014: 11 · 2013: 2
FWCI: 15.82
Type: journal article
Language: en
Open access: closed
Licence: www.elsevier.com/tdm/userlicense/1.0/ (tdm)
Locations: Journal of Hazardous Materials (publishedVersion)
PubMed (publishedVersion)
Funders: National Natural Science Foundation of China (51178321)
National Major Project of Science & Technology Ministry of China (2012ZX07403-001)
Ministry of Housing and Urban-Rural Development (2009-K7-4)
Topics: Physical Sciences › Environmental Science › Water Science and Technology › Advanced oxidation water treatment
Physical Sciences › Environmental Science › Health, Toxicology and Mutagenesis › Water Treatment and Disinfection
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
Keywords: antipyrine, UV/H2O2, UV/persulfate, UV photolysis, advanced oxidation processes, pseudo-first-order kinetics, degradation pathways, emerging contaminants, pharmaceuticals in water, treatment cost comparison, humic acid effects
MeSH terms: Anions, Antipyrine, Bicarbonates, Chlorides, Equipment Design, Humic Substances, Hydrogen Peroxide, Hydrogen-Ion Concentration, Kinetics, Nitrates, Photolysis, Sulfates, Time Factors, Ultraviolet Rays, Water Pollutants, Chemical, Oxidants, Sodium Compounds, Water Purification

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Degradation of antipyrine by UV, UV/H2O2 and UV/PS

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