The DOI matches its Crossref record; 10 of the 10 references it cites were found in a registry or an index.
Carbon Monoxide Gas Diffusion Electrolysis that Produces Concentrated C2 Products with High Single-Pass Conversion
Open accessAbstract
Summary Electrochemical CO conversion is critical for the development of alternative fuel and chemical syntheses. To be efficient, electrosynthesis must make concentrated product streams at high rates with modest potentials, but the combination of these features has not been established for CO or the related CO2 electrolysis. Here we investigate CO electrolysis with gas diffusion electrodes (GDEs) supplied by interdigitated flow fields in electrochemical cells with different ion transport properties. By optimizing gas and ion transport, we show that it is possible to simultaneously achieve high current density, high selectivity, and high single-pass conversion at moderate cell potentials. Using a cell with the GDE directly contacting a Nafion membrane, we demonstrate >100 mA cm−2 CO reduction to C2 products and direct production of 1.1 M acetate at a cell potential of 2.4 V over 24 hr. Our results reveal critical design features for maximizing the efficiency of C2 electrosynthesis.
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How copper catalyzes the electroreduction of carbon dioxide into hydrocarbon fuels
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CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
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Self-citationWhat Should We Make with CO2 and How Can We Make It?
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Technical photosynthesis involving CO2 electrolysis and fermentation
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Probing the Active Surface Sites for CO Reduction on Oxide-Derived Copper Electrocatalysts
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One-step electrosynthesis of ethylene and ethanol from CO2 in an alkaline electrolyzer
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Electrolysis of CO2 to Syngas in Bipolar Membrane-Based Electrochemical Cells
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Cited by
What would it take for renewably powered electrosynthesis to displace petrochemical processes?
De Luna, P., Hahn, C., Higgins, D., Jaffer, S. A., Jaramillo, T. F., & Sargent, E. H. (2019) · Science · doi:10.1126/science.aav3506 · Cited by 3,052
CO 2 electrolysis to multicarbon products in strong acid
Huang, J. E., Li, F., Ozden, A., Sedighian Rasouli, A., García de Arquer, F. P., Liu, S., Zhang, S., Luo, M., Wang, X., Lum, Y., et al. (2021) · Science · doi:10.1126/science.abg6582 · Cited by 1,359
Designing materials for electrochemical carbon dioxide recycling
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Electrocatalytic reduction of CO2 and CO to multi-carbon compounds over Cu-based catalysts
Ma, W., He, X., Wang, W., Xie, S., Zhang, Q., & Wang, Y. (2021) · Chemical Society Reviews · doi:10.1039/d1cs00535a · Cited by 721
Metadata
- Authors
- Ripatti, D. S., Veltman, T. R., & Kanan, M. W.
- Venue
- Joule
- Publisher
- Elsevier BV
- Published
- 2019-01
- Volume
- 3
- Issue
- 1
- Pages
- 240-256
- ISSN
- 2542-4351 (ISSN-L)
- OpenAlex
- W2898431129
- Cited by
- 304
- References
- 10
- FWCI
- 5.77
- Type
- journal article
- Language
- en
- Open access
- bronze
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