Kinetics and mechanism of mineral carbonation of olivine for CO2 sequestration
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The addition of NaHCO3 and NaCl enhances the reactivity of ultramafic mineral phases by retarding the formation of a Si-rich layer around reacted and non-reacted grains.
“The addition of NaHCO3 and NaCl enhances the reactivity of ultramafic mineral phases through retarding the formation of Si-rich layer around the reacted and non-reacted grains36.”
From Low temperature carbonation and CO2 mineral trapping in altered hydrotalcite-rich ultrmafic rocks (2025) · cites this paper as [36]
The reaction comprises three steps: CO2 dissolution generates hydronium ions; hydronium ions attack ultramafic minerals releasing Mg2+ and silicic acid; released Mg2+ reacts with HCO3- and CO3^2- to form nesquehonite.
“This reaction is comprised of three main steps: (1) CO2 dissolution in water generates hydronium ions72; (2) the hydronium ions attack ultramafic minerals resulting in release of Mg2+ ions and formation of silicic acid (H₄SiO4) which either remains in solution or precipitates as amorphous silica36; (3) the released Mg2+ reacts with HCO₃⁻ and carbonate (CO₃²⁻) to form nesquehonite64.”
From Low temperature carbonation and CO2 mineral trapping in altered hydrotalcite-rich ultrmafic rocks (2025) · cites this paper as [36]
The pH buffering effect of the NaHCO3-NaCl solution likely promoted faster dissolution of hydrotalcite compared to other silicate minerals.
“The pH buffering effect of the NaHCO₃–NaCl solution likely promoted faster dissolution of hydrotalcite compared to other silicate minerals36.”
From Low temperature carbonation and CO2 mineral trapping in altered hydrotalcite-rich ultrmafic rocks (2025) · cites this paper as [36]
Incomplete dissolution of both olivine and chrysotile is likely due to formation of silica-layer passivation slowing further dissolution.
“Incomplete dissolution of both olivine and chrysotile is likely due to the formation of silica-layer passivation slowing further dissolution36.”
From Low temperature carbonation and CO2 mineral trapping in altered hydrotalcite-rich ultrmafic rocks (2025) · cites this paper as [36]
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- Authors
- Wang, F., Dreisinger, D., Jarvis, M., & Hitchins, T.
- Affiliations
- University of British Columbia (CA)
- Corresponding author
- Wang, Fei
- Venue
- Minerals Engineering
- Publisher
- Elsevier BV
- Published
- 2019-01
- Volume
- 131
- Pages
- 185-197
- ISSN
- 0892-6875 (ISSN-L)
- OpenAlex
- W2901068949
- Cited by
- 187
- References
- 32
- Citations by year
- 2026: 32 · 2025: 49 · 2024: 38 · 2023: 17 · 2022: 19 · 2021: 15 · 2020: 10 · 2019: 7
- FWCI
- 4.02
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Minerals Engineering (publishedVersion)
- Funders
- Killam
- Natural Sciences and Engineering Research Council of Canada (505580 2016)
- Topics
- Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
- Physical Sciences › Engineering › Mechanical Engineering › Carbon Dioxide Capture Technologies
- Physical Sciences › Chemical Engineering › Process Chemistry and Technology › Carbon dioxide utilization in catalysis
- Keywords
- CO2 mineralization, olivine, CO2 sequestration, carbonation kinetics, reaction mechanism, sodium salts, partial pressure of CO2, particle size effects, temperature effects, bicarbonate, ionic strength, diffusion-controlled reaction, carbonate layers, silica dissolution, amorphous silica, reaction kinetics control
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