Facile preparation of CoNiS/MXene/polypyrrole electrocatalyst with mischcrystal-amorphous interfaces for hydrogen evolution reaction
Open accessAbstract
Electrocatalytic hydrogen evolution reaction (HER) offers a sustainable pathway for clean hydrogen production, while the developing of non-Pt catalysts with high activity and durability remains challenging. This work presents a CoNiS/MXene/polypyrrole (PPy) composite synthesized via a novel 2-step electrodeposition method, enabling precise control over morphology and interfacial properties. The catalyst achieves a low overpotential of 147 mV at 10 mA cm −2 in alkaline media, rivaling state-of-the-art non-Pt HER catalysts. Remarkably, it retains 99% activity after 2000 CV cycles and 12 h of continuous operation, demonstrating exceptional stability. Where, the mischcrystal-amorphous interfaces of CoNiS provides abundant active sites for HER. And the 3D-continuous structure of MXene/PPy offers a large specific surface area and efficient electron-transfer pathways, promoting high-speed charge transport and mass diffusion. The interfacial coupling between CoNiS and the MXene/PPy matrix was considered facilitating efficient charge transfer across their heterojunction interfaces. This interaction effectively prevents the agglomeration and structural degradation of CoNiS nanosheets during the electrocatalytic process, thereby significantly enhancing the stability of the catalyst. The synergistic effects of CoNiS, PPy, and MXene result in an optimized electronic structure and enhanced catalytic kinetics.
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Recent research has focused on other catalysts such as conductive polymers, metal-organic frameworks, and transition metal sulfides with the aim of producing hydrogen efficiently and sustainably.
“Recent research has therefore focused on other catalysts such as conductive polymers, metal-organic frameworks, and transition metal sulfides with the aim of producing hydrogen efficiently and sustainably [47–50].”
From Dual-function aerogel electrocatalyst enabling efficient hydrogen production and ambient-temperature hydrogen detection (2026) · cites this paper as [47]
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- Authors
- Li, H., Su, Y., Guo, T., Zheng, H., Sun, B., Yu, C., Cao, J., Li, Q., & Si, W.
- Affiliations
- Shandong University of Technology (CN)
- Corresponding author
- Si, Weimeng
- Venue
- Next Energy
- Publisher
- Elsevier BV
- Published
- 2025-07
- Volume
- 8
- Pages
- 100338
- ISSN
- 2949-821X (ISSN-L)
- OpenAlex
- W4411992026
- Cited by
- 4
- References
- 93
- Citations by year
- 2026: 4
- FWCI
- 0.56
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Licence
- Locations
- Next Energy (publishedVersion, cc-by)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- Funders
- National Natural Science Foundation of China (21706148)
- Zibo City Integration Development Project (2019ZBXC358)
- Qilu University of Technology State Key Laboratory of Biobased Material and Green Papermaking (KF2019-06)
- Natural Science Foundation of Shandong Province (ZR2020ME041, ZR2022QB173, ZR2023MB054)
- Shandong Academy of Sciences
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Materials Science › Materials Chemistry › Hydrogen Storage and Materials
- Keywords
- hydrogen evolution reaction, electrocatalysts, CONI, MXene, polypyrrole, electrodeposition, heterojunction, charge transfer, catalyst stability, alkaline water electrolysis, hydrogen production
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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