The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Enhanced Nanoparticle Size Control by Extending LaMer’s Mechanism
Open accessAbstract
Abstract The synthesis of well-defined nanoparticle materials has been an area of intense investigation, but size control in nanoparticle syntheses is largely empirical. Here, we introduce a general method for fine size control in the synthesis of nanoparticles by establishing steady state growth conditions through the continuous, controlled addition of precursor, leading to a uniform rate of particle growth. This approach, which we term the “extended LaMer mechanism” allows for reproducibility in particle size from batch to batch as well as the ability to predict nanoparticle size by monitoring the early stages of growth. We have demonstrated this method by applying it to a challenging synthetic system: magnetite nanoparticles. To facilitate this reaction, we have developed a reproducible method for synthesizing an iron oleate precursor that can be used without purification. We then show how such fine size control affects the performance of magnetite nanoparticles in magnetic hyperthermia.
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Citations
Cites
Ultra-large-scale syntheses of monodisperse nanocrystals
Park, J., An, K., Hwang, Y., Park, J.-G., Noh, H.-J., Kim, J.-Y., Park, J.-H., Hwang, N.-M., & Hyeon, T. (2004) · Nature Materials · doi:10.1038/nmat1251 · Cited by 4,076
Theory, Production and Mechanism of Formation of Monodispersed Hydrosols
LaMer, V. K., & Dinegar, R. H. (1950) · Journal of the American Chemical Society · doi:10.1021/ja01167a001 · Cited by 3,894
Colloidal nanocrystal synthesis and the organic–inorganic interface
Yin, Y., & Alivisatos, A. P. (2005) · Nature · doi:10.1038/nature04165 · Cited by 3,273
Monodisperse magnetite nanoparticle tracers for in vivo magnetic particle imaging
Khandhar, A. P., Ferguson, R. M., Arami, H., & Krishnan, K. M. (2013) · Biomaterials · doi:10.1016/j.biomaterials.2013.01.087 · Cited by 152
Cited by
Size-Dependent Heating of Magnetic Iron Oxide Nanoparticles
Tong, S., Quinto, C. A., Zhang, L., Mohindra, P., & Bao, G. (2017) · ACS Nano · doi:10.1021/acsnano.7b01762 · Cited by 401
Metadata
- Authors
- Vreeland, E. C., Watt, J., Schober, G. B., Hance, B. G., Austin, M. J., Price, A. D., Fellows, B. D., Monson, T. C., Hudak, N. S., Maldonado-Camargo, L., Bohorquez, A. C., Rinaldi, C., & Huber, D. L.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-08-21
- Volume
- 27
- Issue
- 17
- Pages
- 6059-6066
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2283296786
- Cited by
- 274
- References
- 4
- FWCI
- 8.39
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- The paper
- Vreeland, E. C., Watt, J., Schober, G. B., Hance, B. G., Austin, M. J., Price, A. D., Fellows, B. D., Monson, T. C., Hudak, N. S., Maldonado-Camargo, L., Bohorquez, A. C., Rinaldi, C., & Huber, D. L. (2015). Enhanced Nanoparticle Size Control by Extending LaMer’s Mechanism. Chemistry of Materials. https://doi.org/10.1021/acs.chemmater.5b02510
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