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Bodipy–Anthracene Dyads as Triplet Photosensitizers: Effect of Chromophore Orientation on Triplet-State Formation Efficiency and Application in Triplet–Triplet Annihilation Upconversion
Abstract
Bodipy-anthracene dyads with two chromophores assuming orthogonal geometry to enhance the spin-orbital charge-transfer intersystem crossing (SOCT-ISC) were prepared. The photosensitizers show strong absorption of visible light, efficient triplet-state formation (quantum yield 90%), and a long-lived triplet state (85 μs). The dipole moment orientation exerts significant effect on the ISC efficiency. It is also the first time that photosensitizers based on SOCT-ISC were used for triplet-triplet annihilation upconversion. The upconversion quantum yield is up to 15.8%.
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Cites
BODIPY dyes in photodynamic therapy
Kamkaew, A., Lim, S. H., Lee, H. B., Kiew, L. V., Chung, L. Y., & Burgess, K. (2013) · Chem. Soc. Rev. · doi:10.1039/c2cs35216h · Cited by 2,104
Fluorescent and luminescent probes for detection of reactive oxygen and nitrogen species
Chen, X., Tian, X., Shin, I., & Yoon, J. (2011) · Chemical Society Reviews · doi:10.1039/c1cs15037e · Cited by 980
Cited by
Wang, C., Chi, W., Qiao, Q., Tan, D., Xu, Z., & Liu, X. (2021) · Chemical Society Reviews · doi:10.1039/d1cs00239b · Cited by 710
Hou, Y., Zhang, X., Chen, K., Liu, D., Wang, Z., Liu, Q., Zhao, J., & Barbon, A. (2019) · Journal of Materials Chemistry C · doi:10.1039/c9tc04285g · Cited by 266
Self-citationNatural Photosensitizers in Antimicrobial Photodynamic Therapy
Polat, E., & Kang, K. (2021) · Biomedicines · doi:10.3390/biomedicines9060584 · Cited by 235
Singlet Oxygen “Afterglow” Therapy with NIR‐II Fluorescent Molecules
Zou, J., Li, L., Zhu, J., Li, X., Yang, Z., Huang, W., & Chen, X. (2021) · Advanced Materials · doi:10.1002/adma.202103627 · Cited by 155
Metadata
- Authors
- Wang, Z., & Zhao, J.
- Venue
- Organic Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-08-15
- Volume
- 19
- Issue
- 17
- Pages
- 4492-4495
- ISSN
- 1523-7052 (ISSN-L)
- 1523-7060
- OpenAlex
- W2749158098
- Cited by
- 203
- References
- 2
- FWCI
- 7.34
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Bodipy–Anthracene Dyads as Triplet Photosensitizers: Effect of Chromophore Orientation on Triplet-State Formation Efficiency and Application in Triplet–Triplet Annihilation Upconversion. https://app.cochat.ai/papers/10.1021/acs.orglett.7b02047
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- Wang, Z., & Zhao, J. (2017). Bodipy–Anthracene Dyads as Triplet Photosensitizers: Effect of Chromophore Orientation on Triplet-State Formation Efficiency and Application in Triplet–Triplet Annihilation Upconversion. Organic Letters. https://doi.org/10.1021/acs.orglett.7b02047
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