The DOI matches its Crossref record; 47 of the 47 references it cites were found in a registry or an index.
Garnet Solid Electrolyte Protected Li-Metal Batteries
Abstract
Garnet-type solid state electrolyte (SSE) is a promising candidate for high performance lithium (Li)-metal batteries due to its good stability and high ionic conductivity. One of the main challenges for garnet solid state batteries is the poor solid–solid contact between the garnet and electrodes, which results in high interfacial resistance, large polarizations, and low efficiencies in batteries. To address this challenge, in this work gel electrolyte is used as an interlayer between solid electrolyte and solid electrodes to improve their contact and reduce their interfacial resistance. The gel electrolyte has a soft structure, high ionic conductivity, and good wettability. Through construction of the garnet/gel interlayer/electrode structure, the interfacial resistance of the garnet significantly decreased from 6.5 × 10 4 to 248 Ω cm 2 for the cathode and from 1.4 × 10 3 to 214 Ω cm 2 for the Li-metal anode, successfully demonstrating a full cell with high capacity (140 mAh/g for LiFePO 4 cathode) over 70 stable cycles in room temperature. This work provides a binary electrolyte consisting of gel electrolyte and solid electrolyte to address the interfacial challenge of solid electrolyte and electrodes and the demonstrated hybrid battery presents a promising future for battery development with high energy and good safety.
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Cites
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Cited by
Interfaces and Interphases in All-Solid-State Batteries with Inorganic Solid Electrolytes
Banerjee, A., Wang, X., Fang, C., Wu, E. A., & Meng, Y. S. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00101 · Cited by 1,526
Gao, Z., Sun, H., Fu, L., Ye, F., Zhang, Y., Luo, W., & Huang, Y. (2018) · Advanced Materials · doi:10.1002/adma.201705702 · Cited by 1,300
Artificial Interphases for Highly Stable Lithium Metal Anode
Xu, R., Cheng, X.-B., Yan, C., Zhang, X.-Q., Xiao, Y., Zhao, C.-Z., Huang, J.-Q., & Zhang, Q. (2019) · Matter · doi:10.1016/j.matt.2019.05.016 · Cited by 721
Liu, W., Liu, P., & Mitlin, D. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202002297 · Cited by 687
Samson, A. J., Hofstetter, K., Bag, S., & Thangadurai, V. (2019) · Energy & Environmental Science · doi:10.1039/c9ee01548e · Cited by 502
Metadata
- Authors
- Liu, B., Gong, Y., Fu, K., Han, X., Yao, Y., Pastel, G., Yang, C., Xie, H., Wachsman, E. D., & Hu, L.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-05-22
- Volume
- 9
- Issue
- 22
- Pages
- 18809-18815
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2613266122
- Cited by
- 287
- References
- 47
- FWCI
- 14.66
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, B., Gong, Y., Fu, K., Han, X., Yao, Y., Pastel, G., Yang, C., Xie, H., Wachsman, E. D., & Hu, L. (2017). Garnet Solid Electrolyte Protected Li-Metal Batteries. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.7b03887
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