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Few-Layered Mo(1–x)WxS2 Hollow Nanospheres on Ni3S2 Nanorod Heterostructure as Robust Electrocatalysts for Overall Water Splitting
Abstract
Owing to unique optical, electronic, and catalytic properties, MoS 2 have received increasing interest in electrochemical water splitting. Herein, few-layered Mo (1-x) W x S 2 hollow nanospheres-modified Ni 3 S 2 heterostructures are prepared through a facile hydrothermal method to further enhance the electrocatalytic performance of MoS 2 . The doping of W element optimizes the electronic structure of MoS 2 @Ni 3 S 2 thus improving the conductivity and charge-transfer ability of MoS 2 @Ni 3 S 2 . In addition, benefitting from the few-layered hollow structure of Mo (1-x) W x S 2 , the strong electronic interactions between Mo (1-x) W x S 2 and Ni 3 S 2 and the hierarchical structure of one-dimensional nanorods and three-dimensional Ni foam, massive active sites and fast ion and charge transportation are obtained. As a result, the optimized Mo (1-x) W x S 2 @Ni 3 S 2 heterostructure (Mo-W-S-2@Ni 3 S 2 ) achieves an extremely low overpotential of 98 mV for hydrogen evolution reaction and 285 mV for oxygen evolution reaction at 10 mA cm -2 in alkaline electrolyte. Particularly, using Mo-W-S-2@Ni 3 S 2 heterostructure as a bifunctional electrocatalyst, a cell voltage of 1.62 V is required to deliver a 10 mA cm -2 water splitting current density. In addition, the electrode can be maintained at 10 mA cm -2 for at least 50 h, indicating the excellent stability of Mo-W-S-2@Ni 3 S 2 heterostructure. Therefore, this development demonstrates an effective and feasible strategy to prepare…
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“Co9S8 is regarded as an attractive material for HER because of its good catalytic activity and stability [24–33].”
From Synthesis of Au/Co9S8 composite aerogels by one-step sol–gel method as hydrogen evolution reaction electrocatalysts (2021) · cites this paper as [33]
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Metadata
- Authors
- Zheng, M., Du, J., Hou, B., & Xu, C.-L.
- Affiliations
- State Key Laboratory of Applied Organic Chemistry (CN)
- Lanzhou No.33 High School, Lanzhou 730000, P. R. China
- State Key Laboratory of Applied Organic Chemistry, Key Laboratory of Nonferrous Metal Chemistry and Resources Utilization of Gansu Province, Laboratory of Special Function Materials and Structure Design of the Ministry of Education, College of Chemistry and Chemical Engineering, Lanzhou University, Lanzhou 730000, P. R. China
- ORCID
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-07-31
- Volume
- 9
- Issue
- 31
- Pages
- 26066-26076
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2736337426
- Cited by
- 136
- References
- 12
- Citations by year
- 2026: 2 · 2025: 5 · 2024: 20 · 2023: 22 · 2022: 10 · 2021: 18 · 2020: 25 · 2019: 16 · 2018: 18
- FWCI
- 4.32
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- ACS Applied Materials & Interfaces (publishedVersion)
- PubMed (publishedVersion)
- Lanzhou University Institutional Repository (submittedVersion)
- Funders
- Ministry of Education of the People's Republic of China (lzujbky-2015-274, lzujbky-2016-K09)
- National Natural Science Foundation of China (21503102, 21673105)
- Key Laboratory of Advanced Energy Materials Chemistry, Nankai University
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
- Keywords
- Ni3S2, heterostructures, hollow nanospheres, nanorods, overall water splitting, bifunctional electrocatalysts, hydrogen evolution reaction, oxygen evolution reaction, tungsten doping, MoS2, nickel foam, alkaline electrolyte, charge transfer, electrocatalyst stability
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