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Engineering NiS/Ni2P Heterostructures for Efficient Electrocatalytic Water Splitting

Xiao, Xin, Huang, Dekang, Fu, Yongqing, Wen, Ming, Jiang, Xingxing, Lv, Xiaowei, Li, Man, Gao, Lin, Liu, Shuangshuang, Wang, Mingkui, Zhao, Chuan, Shen, Yan·2018·ACS Applied Materials & Interfaces

DOI 10.1021/acsami.7b16430

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Abstract

Developing high-active and low-cost bifunctional materials for catalyzing the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) holds a pivotal role in water splitting. Therefore, we present a new strategy to form NiS/Ni 2 P heterostructures. The as-obtained NiS/Ni 2 P/carbon cloth (CC) requires overpotentials of 111 mV for the HER and 265 mV for the OER to reach a current density of 20 mA cm –2, outperforming their counterparts such as NiS and Ni 2 P under the same conditions. Additionally, the NiS/Ni 2 P/CC electrode requires a 1.67 V cell voltage to deliver 10 mA cm –2 in a two-electrode electrolysis system, which is comparable to the cell using the benchmark Pt/C||RuO 2 electrode. Detailed characterizations reveal that strong electronic interactions between NiS and Ni 2 P, abundant active sites, and smaller charge-transfer resistance contribute to the improved HER and OER activity.

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See all 371

Authors: Xiao, X., Huang, D., Fu, Y., Wen, M., Jiang, X., Lv, X., Li, M., Gao, L., Liu, S., Wang, M., Zhao, C., & Shen, Y.
Venue: ACS Applied Materials & Interfaces
Publisher: American Chemical Society (ACS)
Published: 2018-01-23
Volume: 10
Issue: 5
Pages: 4689-4696
ISSN: 1944-8244 (ISSN-L)
1944-8252
DOI: 10.1021/acsami.7b16430
OpenAlex: W2782904998
Cited by: 371
References: 52
FWCI: 10.69
Type: journal article
Language: en
Open access: closed

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Engineering NiS/Ni2P Heterostructures for Efficient Electrocatalytic Water Splitting

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