The DOI matches its Crossref record; 45 of the 45 references it cites were found in a registry or an index.
3D Porous MXene (Ti3C2)/Reduced Graphene Oxide Hybrid Films for Advanced Lithium Storage
Abstract
MXenes, as a new family of 2D materials, can be used as film electrodes in energy storage devices because of their hydrophilic surface, metallic conductivity, and rich surface chemistries. However, the poor ion transport of MXene film electrodes causes a great loss of surface reactivity, which significantly inhibits the full exploitation of the potential of MXene-based materials. To solve this issue, we report a facile electrolyte-induced self-assembly method to construct a 3D porous structure in the MXene–rGO hybrid film, which effectively facilitates rapid diffusion and transport of electrolyte ions in the film electrode while still maintaining high electrical conductivity. When the hybrid film is employed as electrode materials for lithium-ion batteries, it exhibits high specific capacity of 335.5 mA h g –1 at 0.05 A g –1 and good rate capability of 30% capacitance retention at 4 A g –1 . Additionally, the film electrode exhibits excellent cycling stability without capacity decay after 1000 cycles under high rates (1 A g –1 ) owing to its stable structure. Furthermore, the electrochemical analysis also demonstrates that the novel 3D porous microstructure plays an important role in the fast reaction kinetics and high capacity of the MXene–rGO hybrid film electrode. This work may provide a new strategy to solve the issues related to poor ionic transport in MXene-based film electrodes.
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Citations
Cites
Two‐Dimensional Nanocrystals Produced by Exfoliation of Ti3AlC2
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2D metal carbides and nitrides (MXenes) for energy storage
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25th Anniversary Article: MXenes: A New Family of Two‐Dimensional Materials
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Conductive two-dimensional titanium carbide ‘clay’ with high volumetric capacitance
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Two-Dimensional Transition Metal Carbides
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Cation Intercalation and High Volumetric Capacitance of Two-Dimensional Titanium Carbide
Lukatskaya, M. R., Mashtalir, O., Ren, C. E., Dall’Agnese, Y., Rozier, P., Taberna, P. L., Naguib, M., Simon, P., Barsoum, M. W., & Gogotsi, Y. (2013) · Science · doi:10.1126/science.1241488 · Cited by 4,320
Intercalation and delamination of layered carbides and carbonitrides
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Flexible and conductive MXene films and nanocomposites with high capacitance
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Flexible MXene/Graphene Films for Ultrafast Supercapacitors with Outstanding Volumetric Capacitance
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Cited by
Tarcan, R., Todor-Boer, O., Petrovai, I., Leordean, C., Astilean, S., & Botiz, I. (2020) · Journal of Materials Chemistry C · doi:10.1039/c9tc04916a · Cited by 723
Yang, C., Jiang, Q., Li, W., He, H., Yang, L., Lu, Z., & Huang, H. (2019) · Chemistry of Materials · doi:10.1021/acs.chemmater.9b02115 · Cited by 226
Flexible MXene/rGO/CuO hybrid aerogels for high performance acetone sensing at room temperature
Liu, M., Wang, Z., Song, P., Yang, Z., & Wang, Q. (2021) · Sensors and Actuators B: Chemical · doi:10.1016/j.snb.2021.129946 · Cited by 222
Metadata
- Authors
- Ma, Z., Zhou, X., Deng, W., Lei, D., & Liu, Z.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-01-16
- Volume
- 10
- Issue
- 4
- Pages
- 3634-3643
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2782077096
- Cited by
- 389
- References
- 45
- FWCI
- 14.55
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ma, Z., Zhou, X., Deng, W., Lei, D., & Liu, Z. (2018). 3D Porous MXene (Ti3C2)/Reduced Graphene Oxide Hybrid Films for Advanced Lithium Storage. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.7b17386
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