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Incorporation of Imidazolium-Based Poly(ionic liquid)s into a Metal–Organic Framework for CO2 Capture and Conversion
Abstract
The rational integration of multiple functional components into a composite material could result in enhanced activity tailored for specific applications. Herein, imidazolium-based poly(ionic liquid)s (denoted as polyILs) have been confined into the metal–organic framework (MOF) material MIL-101 via in situ polymerization of encapsulated monomers. The resultant composite polyILs@MIL-101 exhibits good CO 2 capture capability that is beneficial for the catalysis of the cycloaddition of CO 2 with epoxides to form cyclic carbonates at subatmospheric pressure in the absence of any cocatalyst. The significantly enhanced activity of polyILs@MIL-101, compared to either MIL-101 or polyILs, is attributed to the synergistic effect among the good CO 2 enrichment capacity, the Lewis acid sites in the MOF, as well as the Lewis base sites in the polyILs.
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Metadata
- Authors
- Ding, M., & Jiang, H.-L.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-03-08
- Volume
- 8
- Issue
- 4
- Pages
- 3194-3201
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2790798973
- Cited by
- 505
- References
- 3
- FWCI
- 16.96
- Type
- journal article
- Language
- en
- Open access
- closed
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