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Dibenzothiophene Dioxide Based Conjugated Microporous Polymers for Visible-Light-Driven Hydrogen Production
Abstract
Conjugated microporous polymers (CMPs) have gained much recent attention as a kind of metal-free organic photocatalyst for photocatalytic hydrogen generation. However, the development of a visible-light-driven CMP photocatalyst with high photocatalytic activity is still a big challenge. Here, we report dibenzothiophene dioxide containing CMP photocatalysts and demonstrate the influence of the cross-linker length on the photocatalytic performance for hydrogen production. The most active photocatalyst of DBTD-CMP1 with a short cross-linker of benzene exhibits a high hydrogen evolution rate (HER) of 2460 μmol h –1 g –1 under visible light without Pt cocatalyst. Remarkably, the Pt-loaded DBTD-CMP1 shows an attractive HER of 9200 μmol h –1 g –1 under UV–vis light illumination. This result demonstrates that these dibenzothiophene dioxide containing CMPs are competitive with the most reported porous organic polymer photocatalysts.
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Cites
Sing, K. S. W. (1985) · Pure and Applied Chemistry · doi:10.1351/pac198557040603 · Cited by 24,485
Cited by
Conjugated polymers for visible-light-driven photocatalysis
Dai, C., & Liu, B. (2020) · Energy & Environmental Science · doi:10.1039/c9ee01935a · Cited by 687
Porous organic polymers: a promising platform for efficient photocatalysis
Zhang, T., Xing, G., Chen, W., & Chen, L. (2020) · Materials Chemistry Frontiers · doi:10.1039/c9qm00633h · Cited by 420
Bai, Y., Wilbraham, L., Slater, B. J., Zwijnenburg, M. A., Sprick, R. S., & Cooper, A. I. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b03591 · Cited by 409
Lan, Z.-A., Ren, W., Chen, X., Zhang, Y., & Wang, X. (2019) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.01.010 · Cited by 265
Conjugated porous polymers: incredibly versatile materials with far-reaching applications
Taylor, D., Dalgarno, S. J., Xu, Z., & Vilela, F. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00315k · Cited by 259
Metadata
- Authors
- Wang, Z., Yang, X., Yang, T., Zhao, Y., Wang, F., Chen, Y., Zeng, J. H., Yan, C., Huang, F., & Jiang, J.-X.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-08-03
- Volume
- 8
- Issue
- 9
- Pages
- 8590-8596
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2885504810
- Cited by
- 263
- References
- 1
- FWCI
- 10.48
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, Z., Yang, X., Yang, T., Zhao, Y., Wang, F., Chen, Y., Zeng, J. H., Yan, C., Huang, F., & Jiang, J.-X. (2018). Dibenzothiophene Dioxide Based Conjugated Microporous Polymers for Visible-Light-Driven Hydrogen Production. ACS Catalysis. https://doi.org/10.1021/acscatal.8b02607
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