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Advances and Promises of Layered Halide Hybrid Perovskite Semiconductors
Open accessAbstract
Layered halide hybrid organic–inorganic perovskites (HOP) have been the subject of intense investigation before the rise of three-dimensional (3D) HOP and their impressive performance in solar cells. Recently, layered HOP have also been proposed as attractive alternatives for photostable solar cells and revisited for light-emitting devices. In this review, we combine classical solid-state physics concepts with simulation tools based on density functional theory to overview the main features of the optoelectronic properties of layered HOP. A detailed comparison between layered and 3D HOP is performed to highlight differences and similarities. In the same way as the cubic phase was established for 3D HOP, here we introduce the tetragonal phase with D 4 h symmetry as the reference phase for 2D monolayered HOP. It allows for detailed analysis of the spin–orbit coupling effects and structural transitions with corresponding electronic band folding. We further investigate the effects of octahedral tilting on the band gap, loss of inversion symmetry and possible Rashba effect, quantum confinement, and dielectric confinement related to the organic barrier, up to excitonic properties. Altogether, this paper aims to provide an interpretive and predictive framework for 3D and 2D layered HOP optoelectronic properties.
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Cites
Self-Consistent Equations Including Exchange and Correlation Effects
Kohn, W., & Sham, L. J. (1965) · Physical Review · doi:10.1103/physrev.140.a1133 · Cited by 64,135
Kim, H.-S., Lee, C.-R., Im, J.-H., Lee, K.-B., Moehl, T., Marchioro, A., Moon, S.-J., Humphry-Baker, R., Yum, J.-H., Moser, J. E., et al. (2012) · Scientific Reports · doi:10.1038/srep00591 · Cited by 8,092
Cited by
Wei, Y., Cheng, Z., & Lin, J. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00740c · Cited by 1,206
Li, X., Hoffman, J. M., & Kanatzidis, M. G. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c01006 · Cited by 1,085
2D Ruddlesden–Popper Perovskites for Optoelectronics
Chen, Y., Sun, Y., Peng, J., Tang, J., Zheng, K., & Liang, Z. (2018) · Advanced Materials · doi:10.1002/adma.201703487 · Cited by 892
Scaling law for excitons in 2D perovskite quantum wells
Blancon, J.-C., Stier, A. V., Tsai, H., Nie, W., Stoumpos, C. C., Traoré, B., Pedesseau, L., Kepenekian, M., Katsutani, F., Noe, G. T., et al. (2018) · Nature Communications · doi:10.1038/s41467-018-04659-x · Cited by 833
Self-citationDu, K.-Z., Tu, Q., Zhang, X., Han, Q., Liu, J., Zauscher, S., & Mitzi, D. B. (2017) · Inorganic Chemistry · doi:10.1021/acs.inorgchem.7b01094 · Cited by 587
Metadata
- Authors
- Pedesseau, L., Sapori, D., Traore, B., Robles, R., Fang, H.-H., Loi, M. A., Tsai, H., Nie, W., Blancon, J.-C., Neukirch, A., Tretiak, S., Mohite, A. D., Katan, C., Even, J., & Kepenekian, M.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-10-24
- Volume
- 10
- Issue
- 11
- Pages
- 9776-9786
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2533429430
- Cited by
- 439
- References
- 2
- FWCI
- 23.17
- Type
- journal article
- Language
- en
- Open access
- green
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- Pedesseau, L., Sapori, D., Traore, B., Robles, R., Fang, H.-H., Loi, M. A., Tsai, H., Nie, W., Blancon, J.-C., Neukirch, A., Tretiak, S., Mohite, A. D., Katan, C., Even, J., & Kepenekian, M. (2016). Advances and Promises of Layered Halide Hybrid Perovskite Semiconductors. ACS Nano. https://doi.org/10.1021/acsnano.6b05944
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