The DOI matches its Crossref record; 32 of the 32 references it cites were found in a registry or an index.
Enhanced Selectivity of MXene Gas Sensors through Metal Ion Intercalation: In Situ X-ray Diffraction Study
Abstract
Gas molecules are known to interact with two-dimensional (2D) materials through surface adsorption where the adsorption-induced charge transfer governs the chemiresistive sensing of various gases. Recently, titanium carbide (Ti 3 C 2 T x ) MXene emerged as a promising sensing channel showing the highest sensitivity among 2D materials and unique gas selectivity. However, unlike conventional 2D materials, MXenes show metallic conductivity and contain interlayer water, implying that gas molecules will likely interact in a more complex way than the typical charge transfer model. Therefore, it is important to understand the role of all factors that may influence gas sensing. Here, we studied the gas-induced interlayer swelling of Ti 3 C 2 T x MXene thin films and its influence on gas sensing performance. In situ X-ray diffraction was employed to simultaneously measure dynamic swelling behavior where Ti 3 C 2 T x MXene films displayed selective swelling toward ethanol vapor over CO 2 gas. Results show that the controlling sodium ion concentration in the interlayers is highly important in tuning the swelling behavior and gas sensing performance. The degree of swelling matched well with the gas response intensity, and the highest gas selectivity toward ethanol vapor was achieved for Ti 3 C 2 T x sensing channels treated with 0.3 mM NaOH, which also displayed the largest amount of swelling. Our results demonstrate that controlling the interlayer transport of Ti 3 C 2 T x MXene is essential for enhancing the selective sensing of gas molecules.
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1 retracted
Hu, M., Hu, T., Li, Z., Yang, Y., Cheng, R., Yang, J., Cui, C., & Wang, X. (2018) · ACS Nano · doi:10.1021/acsnano.8b00676 · Cited by 468
RetractedLipatov, A., Alhabeb, M., Lukatskaya, M. R., Boson, A., Gogotsi, Y., & Sinitskii, A. (2016) · Advanced Electronic Materials · doi:10.1002/aelm.201600255 · Cited by 1,751
Self-citationMetallic Ti3C2T x MXene Gas Sensors with Ultrahigh Signal-to-Noise Ratio
Kim, S. J., Koh, H.-J., Ren, C. E., Kwon, O., Maleski, K., Cho, S.-Y., Anasori, B., Kim, C.-K., Choi, Y.-K., Kim, J., et al. (2018) · ACS Nano · doi:10.1021/acsnano.7b07460 · Cited by 1,699
Self-citationTransparent Conductive Two-Dimensional Titanium Carbide Epitaxial Thin Films
Halim, J., Lukatskaya, M. R., Cook, K. M., Lu, J., Smith, C. R., Näslund, L.-Å., May, S. J., Hultman, L., Gogotsi, Y., Eklund, P., et al. (2014) · Chemistry of Materials · doi:10.1021/cm500641a · Cited by 1,698
Self-citationSemiconducting metal oxides as sensors for environmentally hazardous gases
Wetchakun, K., Samerjai, T., Tamaekong, N., Liewhiran, C., Siriwong, C., Kruefu, V., Wisitsoraat, A., Tuantranont, A., & Phanichphant, S. (2011) · Sensors and Actuators B: Chemical · doi:10.1016/j.snb.2011.08.032 · Cited by 1,241
Atomic Defects in Monolayer Titanium Carbide (Ti3C2Tx) MXene
Sang, X., Xie, Y., Lin, M.-W., Alhabeb, M., Van Aken, K. L., Gogotsi, Y., Kent, P. R. C., Xiao, K., & Unocic, R. R. (2016) · ACS Nano · doi:10.1021/acsnano.6b05240 · Cited by 1,232
Self-citationMXene molecular sieving membranes for highly efficient gas separation
Ding, L., Wei, Y., Li, L., Zhang, T., Wang, H., Xue, J., Ding, L.-X., Wang, S., Caro, J., & Gogotsi, Y. (2018) · Nature Communications · doi:10.1038/s41467-017-02529-6 · Cited by 1,124
Self-citationHanlon, D., Backes, C., Doherty, E., Cucinotta, C. S., Berner, N. C., Boland, C., Lee, K., Harvey, A., Lynch, P., Gholamvand, Z., et al. (2015) · Nature Communications · doi:10.1038/ncomms9563 · Cited by 1,104
Charge- and Size-Selective Ion Sieving Through Ti3C2Tx MXene Membranes
Ren, C. E., Hatzell, K. B., Alhabeb, M., Ling, Z., Mahmoud, K. A., & Gogotsi, Y. (2015) · The Journal of Physical Chemistry Letters · doi:10.1021/acs.jpclett.5b01895 · Cited by 1,030
Self-citationHighly Conductive Optical Quality Solution‐Processed Films of 2D Titanium Carbide
Dillon, A. D., Ghidiu, M. J., Krick, A. L., Griggs, J., May, S. J., Gogotsi, Y., Barsoum, M. W., & Fafarman, A. T. (2016) · Advanced Functional Materials · doi:10.1002/adfm.201600357 · Cited by 988
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Cited by
Ti3C2TX MXene for Sensing Applications: Recent Progress, Design Principles, and Future Perspectives
Pei, Y., Zhang, X., Hui, Z., Zhou, J., Huang, X., Sun, G., & Huang, W. (2021) · ACS Nano · doi:10.1021/acsnano.1c00248 · Cited by 799
Oxidation-resistant titanium carbide MXene films
Lee, Y., Kim, S. J., Kim, Y.-J., Lim, Y., Chae, Y., Lee, B.-J., Kim, Y.-T., Han, H., Gogotsi, Y., & Ahn, C. W. (2020) · Journal of Materials Chemistry A · doi:10.1039/c9ta07036b · Cited by 357
Self-citationYang, Z., Jiang, L., Wang, J., Liu, F., He, J., Liu, A., Lv, S., You, R., Yan, X., Sun, P., et al. (2021) · Sensors and Actuators B: Chemical · doi:10.1016/j.snb.2020.128828 · Cited by 357
Metal-Oxide Nanomaterials Synthesis and Applications in Flexible and Wearable Sensors
Yoon, Y., Truong, P. L., Lee, D., & Ko, S. H. (2022) · ACS Nanoscience Au · doi:10.1021/acsnanoscienceau.1c00029 · Cited by 313
Deshmukh, K., Kovářík, T., & Khadheer Pasha, S. K. (2020) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2020.213514 · Cited by 282
Metadata
- Authors
- Koh, H.-J., Kim, S. J., Maleski, K., Cho, S.-Y., Kim, Y.-J., Ahn, C. W., Gogotsi, Y., & Jung, H.-T.
- Venue
- ACS Sensors
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-05-07
- Volume
- 4
- Issue
- 5
- Pages
- 1365-1372
- ISSN
- 2379-3694 (ISSN-L)
- OpenAlex
- W2944015900
- Cited by
- 257
- References
- 32
- FWCI
- 8.72
- Type
- journal article
- Language
- en
- Open access
- closed
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- Koh, H.-J., Kim, S. J., Maleski, K., Cho, S.-Y., Kim, Y.-J., Ahn, C. W., Gogotsi, Y., & Jung, H.-T. (2019). Enhanced Selectivity of MXene Gas Sensors through Metal Ion Intercalation: In Situ X-ray Diffraction Study. ACS Sensors. https://doi.org/10.1021/acssensors.9b00310
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