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2D ZnIn2S4 Nanosheet/1D TiO2 Nanorod Heterostructure Arrays for Improved Photoelectrochemical Water Splitting
Abstract
We report the fabrication of 2D ZnIn2S4 nanosheet/1D TiO2 nanorod heterojunction arrays by a facile hydrothermal process and their use as photoelectrodes in a photoelectrochemical (PEC) cell for high-performance solar water splitting. The morphology, microstructure, and phase of pristine TiO2 and 2D ZnIn2S4 nanosheet/1D TiO2 nanorod heterojunction arrays were characterized in detail. PEC measurements showed that 2D/1D heterojunction arrays offered enhanced photocurrent density (3 times higher than that of pristine TiO2), negatively shifted onset potential from 0.05 to -0.53 V, and high light on/off cycle stability. Electrochemical impedance investigation attested to a significant improvement of the interface electron transfer kinetics in this heterojunction, thus facilitating electron-hole separation, transfer, and collection, which resulted in enhanced PEC properties.
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Metadata
- Authors
- Liu, Q., Lu, H., Shi, Z., Wu, F., Guo, J., Deng, K., & Li, L.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-09-24
- Volume
- 6
- Issue
- 19
- Pages
- 17200-17207
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2333669114
- Cited by
- 349
- References
- 33
- FWCI
- 7.42
- Type
- journal article
- Language
- en
- Open access
- closed
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