The DOI matches its Crossref record; 32 of the 32 references it cites were found in a registry or an index.
Systematic Investigation of Isoindigo-Based Polymeric Field-Effect Transistors: Design Strategy and Impact of Polymer Symmetry and Backbone Curvature
Abstract
Ten isoindigo-based polymers were synthesized, and their photophysical and electrochemical properties and device performances were systematically investigated. The HOMO levels of the polymers were tuned by introducing different donor units, yet all polymers exhibited p -type semiconducting properties. The hole mobilities of these polymers with centrosymmetric donor units exceeded 0.3 cm 2 V –1 s –1, and the maximum reached 1.06 cm 2 V –1 s –1 . Because of their low-lying HOMO levels, these copolymers also showed good stability upon moisture. AFM and GIXD analyses revealed that polymers with different symmetry and backbone curvature were distinct in lamellar packing and crystallinity. DFT calculations were employed to help us propose the possible packing model. Based on these results, we propose a design strategy, called “molecular docking”, to understand the interpolymer π–π stacking. We also found that polymer symmetry and backbone curvature affect interchain “molecular docking” of isoindigo-based polymers in film, ultimately leading to different device performance. Finally, our design strategy maybe applicable to other reported systems, thus representing a new concept to design conjugated polymers for field-effect transistors.
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Cites
Long-range corrected hybrid density functionals with damped atom–atom dispersion corrections
Chai, J.-D., & Head-Gordon, M. (2008) · Physical Chemistry Chemical Physics · doi:10.1039/b810189b · Cited by 14,648
Charge Transport in Organic Semiconductors
Coropceanu, V., Cornil, J., da Silva Filho, D. A., Olivier, Y., Silbey, R., & Brédas, J.-L. (2007) · Chemical Reviews · doi:10.1021/cr050140x · Cited by 4,607
Docking and scoring in virtual screening for drug discovery: methods and applications
Kitchen, D. B., Decornez, H., Furr, J. R., & Bajorath, J. (2004) · Nature Reviews Drug Discovery · doi:10.1038/nrd1549 · Cited by 4,150
High-Resolution Inkjet Printing of All-Polymer Transistor Circuits
Sirringhaus, H., Kawase, T., Friend, R. H., Shimoda, T., Inbasekaran, M., Wu, W., & Woo, E. P. (2000) · Science · doi:10.1126/science.290.5499.2123 · Cited by 3,311
A high-mobility electron-transporting polymer for printed transistors
Yan, H., Chen, Z., Zheng, Y., Newman, C., Quinn, J. R., Dötz, F., Kastler, M., & Facchetti, A. (2009) · Nature · doi:10.1038/nature07727 · Cited by 3,009
Functionalized Acenes and Heteroacenes for Organic Electronics
Anthony, J. E. (2006) · Chemical Reviews · doi:10.1021/cr050966z · Cited by 2,950
Integrated Optoelectronic Devices Based on Conjugated Polymers
Sirringhaus, H., Tessler, N., & Friend, R. H. (1998) · Science · doi:10.1126/science.280.5370.1741 · Cited by 2,736
Electron and Ambipolar Transport in Organic Field-Effect Transistors
Zaumseil, J., & Sirringhaus, H. (2007) · Chemical Reviews · doi:10.1021/cr0501543 · Cited by 2,197
The Larger Acenes: Versatile Organic Semiconductors
Anthony, J. E. (2008) · Angewandte Chemie International Edition · doi:10.1002/anie.200604045 · Cited by 2,100
All-Polymer Field-Effect Transistor Realized by Printing Techniques
Garnier, F., Hajlaoui, R., Yassar, A., & Srivastava, P. (1994) · Science · doi:10.1126/science.265.5179.1684 · Cited by 1,432
Bronstein, H., Chen, Z., Ashraf, R. S., Zhang, W., Du, J., Durrant, J. R., Shakya Tuladhar, P., Song, K., Watkins, S. E., Geerts, Y., et al. (2011) · Journal of the American Chemical Society · doi:10.1021/ja110619k · Cited by 904
Poly(diketopyrrolopyrrole−terthiophene) for Ambipolar Logic and Photovoltaics
Bijleveld, J. C., Zoombelt, A. P., Mathijssen, S. G. J., Wienk, M. M., Turbiez, M., de Leeuw, D. M., & Janssen, R. A. J. (2009) · Journal of the American Chemical Society · doi:10.1021/ja907506r · Cited by 748
Ultrahigh Mobility in Polymer Field-Effect Transistors by Design
Tsao, H. N., Cho, D. M., Park, I., Hansen, M. R., Mavrinskiy, A., Yoon, D. Y., Graf, R., Pisula, W., Spiess, H. W., & Müllen, K. (2011) · Journal of the American Chemical Society · doi:10.1021/ja108861q · Cited by 705
Reliability of Organic Field‐Effect Transistors
Sirringhaus, H. (2009) · Advanced Materials · doi:10.1002/adma.200901136 · Cited by 618
Functional Organic Field‐Effect Transistors
Guo, Y., Yu, G., & Liu, Y. (2010) · Advanced Materials · doi:10.1002/adma.201000740 · Cited by 585
A High Mobility P‐Type DPP‐Thieno[3,2‐b]thiophene Copolymer for Organic Thin‐Film Transistors
Li, Y., Singh, S. P., & Sonar, P. (2010) · Advanced Materials · doi:10.1002/adma.201002313 · Cited by 546
High-Performance Air-Stable Organic Field-Effect Transistors: Isoindigo-Based Conjugated Polymers
Lei, T., Cao, Y., Fan, Y., Liu, C.-J., Yuan, S.-C., & Pei, J. (2011) · Journal of the American Chemical Society · doi:10.1021/ja111066r · Cited by 485
Self-citationSynthesis of Isoindigo-Based Oligothiophenes for Molecular Bulk Heterojunction Solar Cells
Mei, J., Graham, K. R., Stalder, R., & Reynolds, J. R. (2010) · Organic Letters · doi:10.1021/ol902512x · Cited by 457
High‐Mobility Ambipolar Near‐Infrared Light‐Emitting Polymer Field‐Effect Transistors
Bürgi, L., Turbiez, M., Pfeiffer, R., Bienewald, F., Kirner, H., & Winnewisser, C. (2008) · Advanced Materials · doi:10.1002/adma.200702775 · Cited by 433
Sonar, P., Singh, S. P., Li, Y., Soh, M. S., & Dodabalapur, A. (2010) · Advanced Materials · doi:10.1002/adma.201002973 · Cited by 428
Li, Y., Sonar, P., Singh, S. P., Soh, M. S., van Meurs, M., & Tan, J. (2011) · Journal of the American Chemical Society · doi:10.1021/ja1085996 · Cited by 426
An Easily Accessible Isoindigo-Based Polymer for High-Performance Polymer Solar Cells
Wang, E., Ma, Z., Zhang, Z., Vandewal, K., Henriksson, P., Inganäs, O., Zhang, F., & Andersson, M. R. (2011) · Journal of the American Chemical Society · doi:10.1021/ja206610u · Cited by 373
Conjugated Polymers from Naphthalene Bisimide
Guo, X., & Watson, M. D. (2008) · Organic Letters · doi:10.1021/ol801918y · Cited by 360
Sokolov, A. N., Atahan-Evrenk, S., Mondal, R., Akkerman, H. B., Sánchez-Carrera, R. S., Granados-Focil, S., Schrier, J., Mannsfeld, S. C. B., Zoombelt, A. P., Bao, Z., et al. (2011) · Nature Communications · doi:10.1038/ncomms1451 · Cited by 356
Ha, J. S., Kim, K. H., & Choi, D. H. (2011) · Journal of the American Chemical Society · doi:10.1021/ja203189h · Cited by 347
Novel Thiophene‐Thiazolothiazole Copolymers for Organic Field‐Effect Transistors
Osaka, I., Sauvé, G., Zhang, R., Kowalewski, T., & McCullough, R. D. (2007) · Advanced Materials · doi:10.1002/adma.200701058 · Cited by 305
Chang, J.-F., Clark, J., Zhao, N., Sirringhaus, H., Breiby, D. W., Andreasen, J. W., Nielsen, M. M., Giles, M., Heeney, M., & McCulloch, I. (2006) · Physical Review B · doi:10.1103/physrevb.74.115318 · Cited by 281
Osaka, I., Zhang, R., Sauvé, G., Smilgies, D.-M., Kowalewski, T., & McCullough, R. D. (2009) · Journal of the American Chemical Society · doi:10.1021/ja801475h · Cited by 278
Guo, X., Ortiz, R. P., Zheng, Y., Kim, M.-G., Zhang, S., Hu, Y., Lu, G., Facchetti, A., & Marks, T. J. (2011) · Journal of the American Chemical Society · doi:10.1021/ja205398u · Cited by 238
n-Type Conjugated Polyisoindigos
Stalder, R., Mei, J., Subbiah, J., Grand, C., Estrada, L. A., So, F., & Reynolds, J. R. (2011) · Macromolecules · doi:10.1021/ma2012706 · Cited by 165
Synthesis and Photovoltaic Properties of New Low Bandgap Isoindigo-Based Conjugated Polymers
Zhang, G., Fu, Y., Xie, Z., & Zhang, Q. (2011) · Macromolecules · doi:10.1021/ma102357b · Cited by 153
Highly Stable Semiconducting Polymers Based on Thiazolothiazole
Osaka, I., Zhang, R., Liu, J., Smilgies, D., Kowalewski, T., & McCullough, R. D. (2010) · Chemistry of Materials · doi:10.1021/cm101052b · Cited by 118
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Metadata
- Authors
- Lei, T., Cao, Y., Zhou, X., Peng, Y., Bian, J., & Pei, J.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-05-11
- Volume
- 24
- Issue
- 10
- Pages
- 1762-1770
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2315776551
- Cited by
- 308
- References
- 32
- FWCI
- 26.86
- Type
- journal article
- Language
- en
- Open access
- closed
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