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Hydrogen Generation in Microbial Reverse-Electrodialysis Electrolysis Cells Using a Heat-Regenerated Salt Solution
Abstract
Hydrogen gas can be electrochemically produced in microbial reverse-electrodialysis electrolysis cells (MRECs) using current derived from organic matter and salinity-gradient energy such as river water and seawater solutions. Here, it is shown that ammonium bicarbonate salts, which can be regenerated using low-temperature waste heat, can also produce sufficient voltage for hydrogen gas generation in an MREC. The maximum hydrogen production rate was 1.6 m(3) H(2)/m(3)·d, with a hydrogen yield of 3.4 mol H(2)/mol acetate at a salinity ratio of infinite. Energy recovery was 10% based on total energy applied with an energy efficiency of 22% based on the consumed energy in the reactor. The cathode overpotential was dependent on the catholyte (sodium bicarbonate) concentration, but not the salinity ratio, indicating high catholyte conductivity was essential for maximizing hydrogen production rates. The direction of the HC and LC flows (co- or counter-current) did not affect performance in terms of hydrogen gas volume, production rates, or stack voltages. These results show that the MREC can be successfully operated using ammonium bicarbonate salts that can be regenerated using conventional distillation technologies and waste heat making the MREC a useful method for hydrogen gas production from wastes.
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“Pt-based materials have been the most effective cathode catalysts for MECs;7”
From A 3D hybrid of layered MoS 2 /nitrogen-doped graphene nanosheet aerogels: an effective catalyst for hydrogen evolution in microbial electrolysis cells (2014) · cites this paper as [7]
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Metadata
- Authors
- Nam, J.-Y., Cusick, R. D., Kim, Y., & Logan, B. E.
- Affiliations
- Pennsylvania State University (US)
- Corresponding author
- Logan, Bruce E.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-04-09
- Volume
- 46
- Issue
- 9
- Pages
- 5240-5246
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2101213156
- Cited by
- 105
- References
- 23
- Citations by year
- 2026: 1 · 2025: 3 · 2024: 2 · 2023: 6 · 2022: 12 · 2021: 8 · 2020: 9 · 2019: 6 · 2018: 7 · 2017: 10 · 2016: 10 · 2015: 12 · 2014: 8 · 2013: 6 · 2012: 5
- FWCI
- 8.21
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Environmental Science & Technology (publishedVersion)
- PubMed (publishedVersion)
- King Abdullah University of Science and Technology Repository (King Abdullah University of Science and Technology) (submittedVersion)
- Funders
- King Abdullah University of Science and Technology
- National Renewable Energy Laboratory
- Topics
- Physical Sciences › Environmental Science › Environmental Engineering › Microbial Fuel Cells and Bioremediation
- Physical Sciences › Chemical Engineering › Filtration and Separation › Membrane-based Ion Separation Techniques
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Anaerobic Digestion and Biogas Production
- Keywords
- hydrogen production, waste heat recovery, salinity gradient energy, acetate oxidation, cathodic overpotential, co-current and counter-current flow, energy efficiency, distillation
- MeSH terms
- Bicarbonates, Bioelectric Energy Sources, Hydrogen, Sodium Bicarbonate, Salinity
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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