The DOI matches its Crossref record; 37 of the 37 references it cites were found in a registry or an index.
Sonochemical Degradation of Perfluorooctane Sulfonate (PFOS) and Perfluorooctanoate (PFOA) in Landfill Groundwater: Environmental Matrix Effects
Abstract
Perfluorinated chemicals such as perfluorooctane sulfonate (PFOS) and perfluorooctanoic acid (PFOA) are environmentally persistent and recalcitrant to most conventional chemical and microbial treatment technologies. In this paper, we show that sonolysis is able to decompose PFOS and PFOA present in groundwater beneath a landfill. However, the pseudo first-order rate constant for the sonochemical degradation in the landfill groundwater is reduced by 61 and 56% relative to MilliQ water for PFOS and PFOA, respectively, primarily due to the presence of other organic constituents. In this study, we evaluate the effect of various organic compounds on the sonochemical decomposition rates of PFOS and PFOA. Organic components in environmental matrices may reduce the sonochemical degradation rates of PFOS and PFOA by competitive adsorption onto the bubble-water interface or by lowering the average interfacial temperatures during transient bubble collapse events. The effect of individual organic compounds depends on the Langmuir adsorption constant the Henry's law constant the specific heat capacity, and the overall endothermic heat of dissociation. Volatile organic compounds (VOCs) are identified as the primary cause of the sonochemical rate reduction for PFOS and PFOA in landfill groundwater, whereas the effect of dissolved natural organic matter (DOM) is not significant Finally, a combined process of ozonation and sonolysis is shown to substantially recover the rate loss for PFOS and PFOA in landfill groundwater.
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Citations
Cites
Sources, fate and transport of perfluorocarboxylates
Prevedouros, K., Cousins, I. T., Buck, R. C., & Korzeniowski, S. H. (2006) · Environmental Science & Technology · doi:10.1021/es0512475 · Cited by 2,594
Ellis, D. A., Martin, J. W., De Silva, A. O., Mabury, S. A., Hurley, M. D., Sulbaek Andersen, M. P., & Wallington, T. J. (2004) · Environmental Science & Technology · doi:10.1021/es049860w · Cited by 1,000
A global survey of perfluorinated acids in oceans
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Hori, H., Yamamoto, A., Hayakawa, E., Taniyasu, S., Yamashita, N., Kutsuna, S., Kiatagawa, H., & Arakawa, R. (2005) · Environmental Science & Technology · doi:10.1021/es0484754 · Cited by 595
Mass Loading and Fate of Perfluoroalkyl Surfactants in Wastewater Treatment Plants
Sinclair, E., & Kannan, K. (2006) · Environmental Science & Technology · doi:10.1021/es051798v · Cited by 547
Sonochemical Decomposition of Perfluorooctane Sulfonate and Perfluorooctanoic Acid
Moriwaki, H., Takagi, Y., Tanaka, M., Tsuruho, K., Okitsu, K., & Maeda, Y. (2005) · Environmental Science & Technology · doi:10.1021/es040342v · Cited by 464
Fluorochemical Mass Flows in a Municipal Wastewater Treatment Facility
Schultz, M. M., Higgins, C. P., Huset, C. A., Luthy, R. G., Barofsky, D. F., & Field, J. A. (2006) · Environmental Science & Technology · doi:10.1021/es061025m · Cited by 432
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Perfluorinated Compounds in Coastal Waters of Hong Kong, South China, and Korea
So, M. K., Taniyasu, S., Yamashita, N., Giesy, J. P., Zheng, J., Fang, Z., Im, S. H., & Lam, P. K. S. (2004) · Environmental Science & Technology · doi:10.1021/es049441z · Cited by 402
Cited by
Li, F., Duan, J., Tian, S., Ji, H., Zhu, Y., Wei, Z., & Zhao, D. (2020) · Chemical Engineering Journal · doi:10.1016/j.cej.2019.122506 · Cited by 707
A review of emerging technologies for remediation of PFASs
Ross, I., McDonough, J., Miles, J., Storch, P., Thelakkat Kochunarayanan, P., Kalve, E., Hurst, J., S. Dasgupta, S., & Burdick, J. (2018) · Remediation Journal · doi:10.1002/rem.21553 · Cited by 606
Trojanowicz, M., Bojanowska-Czajka, A., Bartosiewicz, I., & Kulisa, K. (2018) · Chemical Engineering Journal · doi:10.1016/j.cej.2017.10.153 · Cited by 550
Rayne, S., & Forest, K. (2009) · Journal of Environmental Science and Health, Part A · doi:10.1080/10934520903139811 · Cited by 475
Review on the occurrence, fate and removal of perfluorinated compounds during wastewater treatment
Arvaniti, O. S., & Stasinakis, A. S. (2015) · Science of The Total Environment · doi:10.1016/j.scitotenv.2015.04.023 · Cited by 422
Metadata
- Authors
- Cheng, J., Vecitis, C. D., Park, H., Mader, B. T., & Hoffmann, M. R.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-09-23
- Volume
- 42
- Issue
- 21
- Pages
- 8057-8063
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W1996730684
- Cited by
- 277
- References
- 37
- FWCI
- 8.42
- Type
- journal article
- Language
- en
- Open access
- closed
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- Cheng, J., Vecitis, C. D., Park, H., Mader, B. T., & Hoffmann, M. R. (2008). Sonochemical Degradation of Perfluorooctane Sulfonate (PFOS) and Perfluorooctanoate (PFOA) in Landfill Groundwater: Environmental Matrix Effects. Environmental Science & Technology. https://doi.org/10.1021/es8013858
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