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Efficient Removal of Organic Pollutants with Magnetic Nanoscaled BiFeO3 as a Reusable Heterogeneous Fenton-Like Catalyst
Abstract
BiFeO(3) magnetic nanoparticles (BFO MNPs) were prepared with a sol-gel method and characterized as a catalyst. It was found that BFO MNPs effectively catalyzed the decomposition of H(2)O(2) into *OH radicals, being confirmed with electron spin resonance spin-trapping technique and other radical probing techniques. The strong H(2)O(2)-activating ability of BFO MNPs showed promising applications in the oxidative degradation of organic pollutants. When BFO MNPs were used as a heterogeneous Fenton-like catalyst to degrade Rhodamine B, the apparent rate constant for the RhB degradation at 25 degrees C at pH 5.0 in the BFO MNPs-H(2)O(2) system was evaluated to be 2.89 x 10(-2) min(-1), being about 20 folds of that obtained with Fe(3)O(4) MNPs as the catalyst under similar conditions. Moreover, BFO MNPs were demonstrated to have excellent stability and reusability. The catalytic mechanism of BFO MNPs was also investigated with Monte Carlo simulations and density functional theory calculations.
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Cites
Intrinsic peroxidase-like activity of ferromagnetic nanoparticles
Gao, L., Zhuang, J., Nie, L., Zhang, J., Zhang, Y., Gu, N., Wang, T., Feng, J., Yang, D., Perrett, S., et al. (2007) · Nature Nanotechnology · doi:10.1038/nnano.2007.260 · Cited by 7,483
Cited by
Heterogeneous Fenton catalysts: A review of recent advances
Thomas, N., Dionysiou, D. D., & Pillai, S. C. (2021) · Journal of Hazardous Materials · doi:10.1016/j.jhazmat.2020.124082 · Cited by 889
Interfacial mechanisms of heterogeneous Fenton reactions catalyzed by iron-based materials: A review
He, J., Yang, X., Men, B., & Wang, D. (2016) · Journal of Environmental Sciences · doi:10.1016/j.jes.2015.12.003 · Cited by 587
Xin, S., Liu, G., Ma, X., Gong, J., Ma, B., Yan, Q., Chen, Q., Ma, D., Zhang, G., Gao, M., et al. (2021) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2020.119386 · Cited by 567
Zhang, X., Ding, Y., Tang, H., Han, X., Zhu, L., & Wang, N. (2014) · Chemical Engineering Journal · doi:10.1016/j.cej.2013.09.051 · Cited by 465
Self-citationLi, Y., Ouyang, S., Xu, H., Wang, X., Bi, Y., Zhang, Y., & Ye, J. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.6b07272 · Cited by 441
Metadata
- Authors
- Luo, W., Zhu, L., Wang, N., Tang, H., Cao, M., & She, Y.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-02-04
- Volume
- 44
- Issue
- 5
- Pages
- 1786-1791
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2007116337
- Cited by
- 528
- References
- 1
- FWCI
- 25.13
- Type
- journal article
- Language
- en
- Open access
- closed
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- Luo, W., Zhu, L., Wang, N., Tang, H., Cao, M., & She, Y. (2010). Efficient Removal of Organic Pollutants with Magnetic Nanoscaled BiFeO3 as a Reusable Heterogeneous Fenton-Like Catalyst. Environmental Science & Technology. https://doi.org/10.1021/es903390g
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