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Surface-Enhanced Raman Scattering in the Ultraviolet Spectral Region: UV-SERS on Rhodium and Ruthenium Electrodes
Abstract
We report the first observation of surface-enhanced Raman scattering (SERS) excited with ultraviolet (UV) light from transition metal electrodes. Adsorbed pyridine and SCN- on rough rhodium (Rh) and ruthenium (Ru) electrodes, respectively, have been studied using 325 nm laser excitation. In contrast, the best enhancers in the visible and near infrared, silver and gold, do not produce UV-SERS. The experimental data of UV-SERS are in agreement with our preliminary theoretical calculation based on the electromagnetic enhancement mechanism. The enhancement factor is about 2 orders of magnitude for the Rh and Ru electrodes when they are excited at 325 nm.
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Toward a Glucose Biosensor Based on Surface-Enhanced Raman Scattering
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Cited by
Electromagnetic Mechanism of SERS
Schatz, G. C., Young, M. A., & Duyne, R. P. (2006) · Topics in Applied Physics · doi:10.1007/3-540-33567-6_2 · Cited by 469
Tip-Enhanced Raman Spectroscopy: Technique and Recent Advances
Verma, P. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00821 · Cited by 448
Surface-enhanced Raman spectroscopy: a half-century historical perspective
Yi, J., You, E.-M., Hu, R., Wu, D.-Y., Liu, G.-K., Yang, Z.-L., Zhang, H., Gu, Y., Wang, Y.-H., Wang, X., et al. (2025) · Chemical Society Reviews · doi:10.1039/d4cs00883a · Cited by 382
Self-citationNanoparticles Engineering by Pulsed Laser Ablation in Liquids: Concepts and Applications
Fazio, E., Gökce, B., De Giacomo, A., Meneghetti, M., Compagnini, G., Tommasini, M., Waag, F., Lucotti, A., Zanchi, C. G., Ossi, P. M., et al. (2020) · Nanomaterials · doi:10.3390/nano10112317 · Cited by 346
Deep-UV surface-enhanced Raman scattering
Dörfer, T., Schmitt, M., & Popp, J. (2007) · Journal of Raman Spectroscopy · doi:10.1002/jrs.1831 · Cited by 141
Metadata
- Authors
- Ren, B., Lin, X.-F., Yang, Z.-L., Liu, G.-K., Aroca, R. F., Mao, B.-W., & Tian, Z.-Q.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2003-07-19
- Volume
- 125
- Issue
- 32
- Pages
- 9598-9599
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2079991227
- Cited by
- 217
- References
- 1
- FWCI
- 5.51
- Type
- journal article
- Language
- en
- Open access
- closed
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