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Unidirectional Electronic Ring Current Driven by a Few Cycle Circularly Polarized Laser Pulse: Quantum Model Simulations for Mg−Porphyrin
Abstract
A circularly polarized ultraviolet (UV) laser pulse may excite a unidirectional valence-type electronic ring current in an oriented molecule, within the pulse duration of a few femtoseconds (e.g., tau = 3.5 fs). The mechanism is demonstrated by quantum model simulation for |X = |1(1)A(1g) --> |E(+) = |4 (1)E(u+) population transfer in the model system, Mg-porphyrin. The net ring current generated by the laser pulse (I = 84.5 microA) is at least 100 times stronger than any ring current, which could be induced by means of permanent magnetic fields, with present technology.
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Metadata
- Authors
- Barth, I., Manz, J., Shigeta, Y., & Yagi, K.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-05-01
- Volume
- 128
- Issue
- 21
- Pages
- 7043-7049
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2008006945
- Cited by
- 269
- References
- 29
- FWCI
- 9.02
- Type
- journal article
- Language
- en
- Open access
- closed
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