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Electocatalytic Water Oxidation by Cobalt(III) Hangman β-Octafluoro Corroles
Abstract
Cobalt hangman corrole, bearing β-octafluoro and meso-pentafluorophenyl substituents, is an active water splitting catalyst. When immobilized in Nafion films, the turnover frequencies for the 4e(-)/4H(+) process at the single cobalt center of the hangman platform approach 1 s(-1). The pH dependence of the water splitting reaction suggests a proton-coupled electron transfer (PCET) catalytic mechanism.
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Metadata
- Authors
- Dogutan, D. K., McGuire, R., & Nocera, D. G.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-05-27
- Volume
- 133
- Issue
- 24
- Pages
- 9178-9180
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2333596353
- Cited by
- 525
- References
- 0
- FWCI
- 16.29
- Type
- journal article
- Language
- en
- Open access
- closed
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