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A Solid Lithium Electrolyte via Addition of Lithium Isopropoxide to a Metal–Organic Framework with Open Metal Sites
Abstract
The uptake of LiO(i)Pr in Mg(2)(dobdc) (dobdc(4-) = 1,4-dioxido-2,5-benzenedicarboxylate) followed by soaking in a typical electrolyte solution leads to the new solid lithium electrolyte Mg(2)(dobdc)·0.35LiO(i)Pr·0.25LiBF(4)·EC·DEC (EC = ethylene carbonate; DEC = diethyl carbonate). Two-point ac impedance data show a pressed pellet of this material to have a conductivity of 3.1 × 10(-4) S/cm at 300 K. In addition, the results from variable-temperature measurements reveal an activation energy of just 0.15 eV, while single-particle data suggest that intraparticle transport dominates conduction.
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Metadata
- Authors
- Wiers, B. M., Foo, M.-L., Balsara, N. P., & Long, J. R.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-08-30
- Volume
- 133
- Issue
- 37
- Pages
- 14522-14525
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2024540372
- Cited by
- 454
- References
- 46
- FWCI
- 9.80
- Type
- journal article
- Language
- en
- Open access
- closed
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