The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Diffusion Mechanism of Lithium Ion through Basal Plane of Layered Graphene
Abstract
Coexistence of both edge plane and basal plane in graphite often hinders the understanding of lithium ion diffusion mechanism. In this report, two types of graphene samples were prepared by chemical vapor deposition (CVD): (i) well-defined basal plane graphene grown on Cu foil and (ii) edge plane-enriched graphene layers grown on Ni film. Electrochemical performance of the graphene electrode can be split into two regimes depending on the number of graphene layers: (i) the corrosion-dominant regime and (ii) the lithiation-dominant regime. Li ion diffusion perpendicular to the basal plane of graphene is facilitated by defects, whereas diffusion parallel to the plane is limited by the steric hindrance that originates from aggregated Li ions adsorbed on the abundant defect sites. The critical layer thickness (l(c)) to effectively prohibit substrate reaction using CVD-grown graphene layers was predicted to be ∼6 layers, independent of defect population. Our density functional theory calculations demonstrate that divacancies and higher order defects have reasonable diffusion barrier heights allowing lithium diffusion through the basal plane but neither monovacancies nor Stone-Wales defect.
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Cites
Fine Structure Constant Defines Visual Transparency of Graphene
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Ageing mechanisms in lithium-ion batteries
Vetter, J., Novák, P., Wagner, M. R., Veit, C., Möller, K.-C., Besenhard, J. O., Winter, M., Wohlfahrt-Mehrens, M., Vogler, C., & Hammouche, A. (2005) · Journal of Power Sources · doi:10.1016/j.jpowsour.2005.01.006 · Cited by 3,987
Capacity Fade Mechanisms and Side Reactions in Lithium‐Ion Batteries
Arora, P., White, R. E., & Doyle, M. (1998) · Journal of The Electrochemical Society · doi:10.1149/1.1838857 · Cited by 1,408
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Chang, J., Jin, M., Yao, F., Kim, T. H., Le, V. T., Yue, H., Gunes, F., Li, B., Ghosh, A., Xie, S., et al. (2013) · Advanced Functional Materials · doi:10.1002/adfm201301851 · Cited by 707
Self-citationFast Charging Anode Materials for Lithium‐Ion Batteries: Current Status and Perspectives
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Lin, X., Khosravinia, K., Hu, X., Li, J., & Lu, W. (2021) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2021.100953 · Cited by 490
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Chen, K., Song, S., Liu, F., & Xue, D. (2015) · Chemical Society Reviews · doi:10.1039/c5cs00147a · Cited by 446
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Various defects in graphene: a review
Bhatt, M. D., Kim, H., & Kim, G. (2022) · RSC Advances · doi:10.1039/d2ra01436j · Cited by 386
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Self-citation
Metadata
- Authors
- Yao, F., Güneş, F., Ta, H. Q., Lee, S. M., Chae, S. J., Sheem, K. Y., Cojocaru, C. S., Xie, S. S., & Lee, Y. H.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-05-11
- Volume
- 134
- Issue
- 20
- Pages
- 8646-8654
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2013457020
- Cited by
- 401
- References
- 3
- FWCI
- 13.63
- Type
- journal article
- Language
- en
- Open access
- closed
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