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A Series of Highly Stable Mesoporous Metalloporphyrin Fe-MOFs
Abstract
A series of mesoporous metalloporphyrin Fe-MOFs, namely PCN-600(M) (M = Mn, Fe, Co, Ni, Cu), have been synthesized using the preassembled [Fe3O(OOCCH3)6] building block. PCN-600 exhibits a one-dimensional channel as large as 3.1 nm and the highest experimental pore volume of 1.80 cm(3)g(-1) among all the reported porphyrinic MOFs. It also shows very high stability in aqueous solutions with pH values ranging from 2-11 and is to our knowledge the only mesoporous porphyrinic MOF stable under basic aqueous conditions. PCN-600(Fe) has been demonstrated as an effective peroxidase mimic to catalyze the co-oxidation reaction.
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Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
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Best Practices for the Synthesis, Activation, and Characterization of Metal–Organic Frameworks
Howarth, A. J., Peters, A. W., Vermeulen, N. A., Wang, T. C., Hupp, J. T., & Farha, O. K. (2017) · Chemistry of Materials · doi:10.1021/acs.chemmater.6b02626 · Cited by 746
Metal–organic frameworks (MOFs) for the removal of emerging contaminants from aquatic environments
Dhaka, S., Kumar, R., Deep, A., Kurade, M. B., Ji, S.-W., & Jeon, B.-H. (2019) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2018.10.003 · Cited by 615
Bioinspired Framework Catalysts: From Enzyme Immobilization to Biomimetic Catalysis
Wang, K.-Y., Zhang, J., Hsu, Y.-C., Lin, H., Han, Z., Pang, J., Yang, Z., Liang, R.-R., Shi, W., & Zhou, H.-C. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00879 · Cited by 490
Self-citationConstruction and application of base-stable MOFs: a critical review
Wang, K., Li, Y., Xie, L.-H., Li, X., & Li, J.-R. (2022) · Chemical Society Reviews · doi:10.1039/d1cs00891a · Cited by 462
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Metadata
- Authors
- Wang, K., Feng, D., Liu, T.-F., Su, J., Yuan, S., Chen, Y.-P., Bosch, M., Zou, X., & Zhou, H.-C.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-09-23
- Volume
- 136
- Issue
- 40
- Pages
- 13983-13986
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2064804729
- Cited by
- 452
- References
- 1
- FWCI
- 13.40
- Type
- journal article
- Language
- en
- Open access
- closed
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