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Highly Active and Selective Hydrogenation of CO2 to Ethanol by Ordered Pd–Cu Nanoparticles
Abstract
Carbon dioxide (CO 2 ) hydrogenation to ethanol (C 2 H 5 OH) is considered a promising way for CO 2 conversion and utilization, whereas desirable conversion efficiency remains a challenge. Herein, highly active, selective and stable CO 2 hydrogenation to C 2 H 5 OH was enabled by highly ordered Pd-Cu nanoparticles (NPs). By tuning the composition of the Pd-Cu NPs and catalyst supports, the efficiency of CO 2 hydrogenation to C 2 H 5 OH was well optimized with Pd 2 Cu NPs/P25 exhibiting high selectivity to C 2 H 5 OH of up to 92.0% and the highest turnover frequency of 359.0 h –1 . Diffuse reflectance infrared Fourier transform spectroscopy results revealed the high C 2 H 5 OH production and selectivity of Pd 2 Cu NPs/P25 can be ascribed to boosting *CO (adsorption CO) hydrogenation to *HCO, the rate-determining step for the CO 2 hydrogenation to C 2 H 5 OH.
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Cites
Recent advances in catalytic hydrogenation of carbon dioxide
Wang, W., Wang, S., Ma, X., & Gong, J. (2011) · Chemical Society Reviews · doi:10.1039/c1cs15008a · Cited by 3,316
He, Z., Qian, Q., Ma, J., Meng, Q., Zhou, H., Song, J., Liu, Z., & Han, B. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201507585 · Cited by 313
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The renaissance of the Sabatier reaction and its applications on Earth and in space.
Vogt, C., Monai, M., Kramer, G. J., & Weckhuysen, B. M. (2019) · Nature Catalysis · doi:10.1038/s41929-019-0244-4 · Cited by 636
Direct Production of Lower Olefins from CO2 Conversion via Bifunctional Catalysis
Gao, P., Dang, S., Li, S., Bu, X., Liu, Z., Qiu, M., Yang, C., Wang, H., Zhong, L., Han, Y., et al. (2018) · ACS Catalysis · doi:10.1021/acscatal.7b02649 · Cited by 533
Selective Hydrogenation of CO2 to Ethanol over Cobalt Catalysts
Wang, L., Wang, L., Zhang, J., Liu, X., Wang, H., Zhang, W., Yang, Q., Ma, J., Dong, X., Yoo, S. J., et al. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201800729 · Cited by 389
Significant Advances in C1 Catalysis: Highly Efficient Catalysts and Catalytic Reactions
Bao, J., Yang, G., Yoneyama, Y., & Tsubaki, N. (2019) · ACS Catalysis · doi:10.1021/acscatal.8b03924 · Cited by 367
Huang, H., Chen, C., Chang, C., Lai, F., Liu, S., Fu, H., Chen, Y., Li, H., Huang, W., Zhang, N., et al. (2024) · Advanced Materials · doi:10.1002/adma.202314142 · Cited by 40
Metadata
- Authors
- Bai, S., Shao, Q., Wang, P., Dai, Q., Wang, X., & Huang, X.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-05-15
- Volume
- 139
- Issue
- 20
- Pages
- 6827-6830
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2613395675
- Cited by
- 487
- References
- 2
- FWCI
- 12.76
- Type
- journal article
- Language
- en
- Open access
- closed
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- Bai, S., Shao, Q., Wang, P., Dai, Q., Wang, X., & Huang, X. (2017). Highly Active and Selective Hydrogenation of CO2 to Ethanol by Ordered Pd–Cu Nanoparticles. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.7b03101
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