The DOI matches its Crossref record; 27 of the 27 references it cites were found in a registry or an index.
Selective Hydrogenation of CO2 to Ethanol over Cobalt Catalysts
Abstract
Methods for the hydrogenation of CO 2 into valuable chemicals are in great demand but their development is still challenging. Herein, we report the selective hydrogenation of CO 2 into ethanol over non‐noble cobalt catalysts (CoAlOx), presenting a significant advance for the conversion of CO 2 into ethanol as the major product. By adjusting the composition of the catalysts through the use of different prereduction temperatures, the efficiency of CO 2 to ethanol hydrogenation was optimized; the catalyst reduced at 600 ° gave an ethanol selectivity of 92.1 % at 140 °C with an ethanol time yield of 0.444 mmol g−1 h−1. Operando FT‐IR spectroscopy revealed that the high ethanol selectivity over the CoAlOx catalyst might be due to the formation of acetate from formate by insertion of *CHx, a key intermediate in the production of ethanol by CO 2 hydrogenation.
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Cites
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Cited by
Industrial carbon dioxide capture and utilization: state of the art and future challenges
Gao, W., Liang, S., Wang, R., Jiang, Q., Zhang, Y., Zheng, Q., Xie, B., Toe, C. Y., Zhu, X., Wang, J., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00025f · Cited by 1,388
Self-citationSignificant Advances in C1 Catalysis: Highly Efficient Catalysts and Catalytic Reactions
Bao, J., Yang, G., Yoneyama, Y., & Tsubaki, N. (2019) · ACS Catalysis · doi:10.1021/acscatal.8b03924 · Cited by 367
Belthle, K. S., Beyazay, T., Ochoa-Hernández, C., Miyazaki, R., Foppa, L., Martin, W. F., & Tüysüz, H. (2022) · Journal of the American Chemical Society · doi:10.1021/jacs.2c08845 · Cited by 41
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Pamei, M., Sharma, S. K., Das, D., Vadivel, S., Paul, B., & Puzari, A. (2026) · Catalysis Reviews · doi:10.1080/01614940.2024.2400974 · Cited by 11
Metadata
- Authors
- Wang, L., Wang, L., Zhang, J., Liu, X., Wang, H., Zhang, W., Yang, Q., Ma, J., Dong, X., Yoo, S. J., Kim, J., Meng, X., & Xiao, F.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-04-25
- Volume
- 57
- Issue
- 21
- Pages
- 6104-6108
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2802735530
- Cited by
- 389
- References
- 27
- FWCI
- 7.30
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, L., Wang, L., Zhang, J., Liu, X., Wang, H., Zhang, W., Yang, Q., Ma, J., Dong, X., Yoo, S. J., Kim, J., Meng, X., & Xiao, F. (2018). Selective Hydrogenation of CO2 to Ethanol over Cobalt Catalysts. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201800729
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