The DOI matches its Crossref record; 23 of the 23 references it cites were found in a registry or an index.
Metal–Organic Framework Coating Enhances the Performance of Cu2O in Photoelectrochemical CO2 Reduction
Abstract
Photoelectrochemical (PEC) reduction of CO 2 into chemical fuels and chemical building blocks is a promising strategy for addressing the energy and environmental challenges, which relies on the development of p-type photocathodes. Cu 2 O is such a p-type semiconductor for photocathodes but commonly suffers from detrimental photocorrosion and chemical changes. In this communication, we develop a facile procedure for coating a metal–organic framework (MOF) on the surface of a Cu 2 O photocathode, which can both prevent photocorrosion and offer active sites for CO 2 reduction. As evidenced by ultrafast spectroscopy, the formed interface can effectively promote charge separation and transfer. As a result, both the activity and durability of Cu 2 O are dramatically enhanced for PEC CO 2 reduction. This work provides fresh insights into the design of advanced hybrid photoelectrodes and highlights the important role of interfacial charge dynamics in PEC CO 2 conversion.
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Cites
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Industrial carbon dioxide capture and utilization: state of the art and future challenges
Gao, W., Liang, S., Wang, R., Jiang, Q., Zhang, Y., Zheng, Q., Xie, B., Toe, C. Y., Zhu, X., Wang, J., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00025f · Cited by 1,388
Self-citationYan, Y., Li, C., Wu, Y., Gao, J., & Zhang, Q. (2020) · Journal of Materials Chemistry A · doi:10.1039/d0ta03749d · Cited by 260
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Metadata
- Authors
- Deng, X., Li, R., Wu, S., Wang, L., Hu, J., Ma, J., Jiang, W., Zhang, N., Zheng, X., Gao, C., Wang, L., Zhang, Q., Zhu, J., & Xiong, Y.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-06-14
- Volume
- 141
- Issue
- 27
- Pages
- 10924-10929
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2951075750
- Cited by
- 322
- References
- 23
- FWCI
- 7.83
- Type
- journal article
- Language
- en
- Open access
- closed
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- Deng, X., Li, R., Wu, S., Wang, L., Hu, J., Ma, J., Jiang, W., Zhang, N., Zheng, X., Gao, C., Wang, L., Zhang, Q., Zhu, J., & Xiong, Y. (2019). Metal–Organic Framework Coating Enhances the Performance of Cu2O in Photoelectrochemical CO2 Reduction. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.9b06239
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