The DOI matches its Crossref record; 14 of the 14 references it cites were found in a registry or an index.
ζ Potential of Microbubbles in Aqueous Solutions: Electrical Properties of the Gas−Water Interface
Abstract
Microbubbles are very fine bubbles and appropriate for the investigation of the gas-water interface electrical charge, because of their long stagnation, due to slow buoyancy, in the electrophoresis cell observation area. This study investigated the zeta potential of microbubbles in aqueous solutions and revealed that the bubbles were negatively charged under a wide range of pH conditions. The potential was positive under strong acidic conditions, and the inorganic electrolytes decrease the potential by increasing the amount of counterions within the slipping plane. OH(-) and H(+) are crucial factors for the charging mechanism of the gas-water interface, while other anions and cations have secondary effects on the zeta potential, because counterions are attracted by the interface charge. The addition of a small amount of propanol and butanol provided significant information for considering the mechanism of the gas-water interface charge. Even though these alcohols did not have any electrical charge, they had a strong effect on the gas-water interface charge and dispersed the zeta potential of the microbubbles in the aqueous solution. These alcohols tended to adsorb to the interface and affect the hydrogen-bonding network at the interface, so that it was concluded that the gas-water interface electrical charge must be related to the difference of the construction of the hydrogen-bonding network between the bulk water and the gas-water interface.
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Citations
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Protons and Hydroxide Ions in Aqueous Systems
Agmon, N., Bakker, H. J., Campen, R. K., Henchman, R. H., Pohl, P., Roke, S., Thämer, M., & Hassanali, A. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00736 · Cited by 538
Meegoda, J. N., Aluthgun Hewage, S., & Batagoda, J. H. (2018) · Environmental Engineering Science · doi:10.1089/ees.2018.0203 · Cited by 294
Gas Evolution in Water Electrolysis
Kempler, P. A., Coridan, R. H., & Luo, L. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.4c00211 · Cited by 289
The Orientation and Charge of Water at the Hydrophobic Oil Droplet–Water Interface
Vácha, R., Rick, S. W., Jungwirth, P., de Beer, A. G. F., de Aguiar, H. B., Samson, J.-S., & Roke, S. (2011) · Journal of the American Chemical Society · doi:10.1021/ja202081x · Cited by 278
Hydroxide and hydronium ion adsorption — A survey
Zimmermann, R., Freudenberg, U., Schweiß, R., Küttner, D., & Werner, C. (2010) · Current Opinion in Colloid & Interface Science · doi:10.1016/j.cocis.2010.01.002 · Cited by 261
Metadata
- Authors
- Takahashi, M.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 2005-10-29
- Volume
- 109
- Issue
- 46
- Pages
- 21858-21864
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W1997295143
- Cited by
- 888
- References
- 14
- FWCI
- 14.64
- Type
- journal article
- Language
- en
- Open access
- closed
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