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Tetraalkylphosphonium Polyoxometalate Ionic Liquids: Novel, Organic−Inorganic Hybrid Materials
Abstract
Pairing of a Keggin or Lindqvist polyoxometalate (POM) anion with an appropriate tetraalkylphosphonium cation is shown to yield the first members of a new family of ionic liquids (ILs). Detailed characterization of one of them, an ambient-temperature "liquid POM" comprising the Lindqvist salt of the trihexyl(tetradecyl) phosphonium cation, by voltammetry, viscometry, conductimetry, and thermal analysis indicates that it exhibits conductivity and viscosity comparable to those of the one previously described inorganic-organic POM-IL hybrid but with substantially improved thermal stability.
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Citations
Cites
Ionic liquids: solvent properties and organic reactivity
Chiappe, C., & Pieraccini, D. (2005) · Journal of Physical Organic Chemistry · doi:10.1002/poc.863 · Cited by 1,169
Application of ionic liquids to the electrodeposition of metals
Abbott, A. P., & McKenzie, K. J. (2006) · Physical Chemistry Chemical Physics · doi:10.1039/b607329h · Cited by 817
Thermal Degradation of Ionic Liquids at Elevated Temperatures
Baranyai, K. J., Deacon, G. B., MacFarlane, D. R., Pringle, J. M., & Scott, J. L. (2004) · Australian Journal of Chemistry · doi:10.1071/ch03221 · Cited by 338
Cited by
Beyond Charge Balance: Counter‐Cations in Polyoxometalate Chemistry
Misra, A., Kozma, K., Streb, C., & Nyman, M. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201905600 · Cited by 482
Semimetal-functionalised polyoxovanadates
Monakhov, K. Y., Bensch, W., & Kögerler, P. (2015) · Chemical Society Reviews · doi:10.1039/c5cs00531k · Cited by 290
Metadata
- Authors
- Rickert, P. G., Antonio, M. R., Firestone, M. A., Kubatko, K.-A., Szreder, T., Wishart, J. F., & Dietz, M. L.
- Venue
- The Journal of Physical Chemistry B
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-05-01
- Volume
- 111
- Issue
- 18
- Pages
- 4685-4692
- ISSN
- 1520-5207 (ISSN-L)
- 1520-6106
- OpenAlex
- W1982270483
- Cited by
- 166
- References
- 3
- FWCI
- 3.77
- Type
- journal article
- Language
- en
- Open access
- closed
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- Rickert, P. G., Antonio, M. R., Firestone, M. A., Kubatko, K.-A., Szreder, T., Wishart, J. F., & Dietz, M. L. (2007). Tetraalkylphosphonium Polyoxometalate Ionic Liquids: Novel, Organic−Inorganic Hybrid Materials. The Journal of Physical Chemistry B. https://doi.org/10.1021/jp0671751
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