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The Effects of Crystal Structure and Electronic Structure on Photocatalytic H2 Evolution and CO2 Reduction over Two Phases of Perovskite-Structured NaNbO3
Open accessAbstract
Cubic and orthorhombic NaNbO 3 were fabricated to study the effects of crystal structure and electronic structure on the photocatalytic activities in detail. The samples were characterized by X-ray diffraction, field emission transmission electron microscopy, high-resolution transmission electron microscopy, UV–visible absorption spectroscopy, and X-ray photoelectron spectroscopy. The photocatalytic activities of the two phases of NaNbO 3 have been assessed by H 2 evolution from aqueous methanol solution and CO 2 photoreduction in gas phase. The photocatalytic H 2 evolution and CO 2 reduction activities over cubic NaNbO 3 were nearly twice of those over orthorhombic NaNbO 3 . The first-principles calculation reveals that the higher activity over cubic NaNbO 3 can be attributed to its unique electronic structure, which is beneficial for electron excitation and transfer.
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Metadata
- Authors
- Li, P., Ouyang, S., Xi, G., Kako, T., & Ye, J.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-03-26
- Volume
- 116
- Issue
- 14
- Pages
- 7621-7628
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W1995506895
- Cited by
- 277
- References
- 34
- FWCI
- 7.65
- Type
- journal article
- Language
- en
- Open access
- green
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