The DOI matches its Crossref record; 17 of the 17 references it cites were found in a registry or an index.
High Electrochemical Selectivity of Edge versus Terrace Sites in Two-Dimensional Layered MoS2 Materials
Abstract
Exploring the chemical reactivity of different atomic sites on crystal surface and controlling their exposures are important for catalysis and renewable energy storage. Here, we use two-dimensional layered molybdenum disulfide (MoS2) to demonstrate the electrochemical selectivity of edge versus terrace sites for Li-S batteries and hydrogen evolution reaction (HER). Lithium sulfide (Li2S) nanoparticles decorates along the edges of the MoS2 nanosheet versus terrace, confirming the strong binding energies between Li2S and the edge sites and guiding the improved electrode design for Li-S batteries. We also provided clear comparison of HER activity between edge and terrace sites of MoS2 beyond the previous theoretical prediction and experimental proof.
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Cited by
Voiry, D., Yang, J., & Chhowalla, M. (2016) · Advanced Materials · doi:10.1002/adma.201505597 · Cited by 949
Yu, P., Wang, F., Shifa, T. A., Zhan, X., Lou, X., Xia, F., & He, J. (2019) · Nano Energy · doi:10.1016/j.nanoen.2019.01.017 · Cited by 434
Liu, W., Luo, C., Zhang, S., Zhang, B., Ma, J., Wang, X., Liu, W., Li, Z., Yang, Q.-H., & Lv, W. (2021) · ACS Nano · doi:10.1021/acsnano.1c00896 · Cited by 269
Face the Edges: Catalytic Active Sites of Nanomaterials
Ni, B., & Wang, X. (2015) · Advanced Science · doi:10.1002/advs.201500085 · Cited by 219
Li, G., Chen, Z., Li, Y., Zhang, D., Yang, W., Liu, Y., & Cao, L. (2020) · ACS Nano · doi:10.1021/acsnano.9b07324 · Cited by 147
Metadata
- Authors
- Wang, H., Zhang, Q., Yao, H., Liang, Z., Lee, H.-W., Hsu, P.-C., Zheng, G., & Cui, Y.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-11-10
- Volume
- 14
- Issue
- 12
- Pages
- 7138-7144
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2335721177
- Cited by
- 312
- References
- 17
- FWCI
- 6.33
- Type
- journal article
- Language
- en
- Open access
- closed
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