Cited by 481Graphene research and applicationsCarbon Nanotubes in CompositesCarbon and Quantum Dots Applications

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Brightening of carbon nanotube photoluminescence through the incorporation of sp3 defects

Piao, Yanmei, Meany, Brendan, Powell, Lyndsey R., Valley, Nicholas, Kwon, Hyejin, Schatz, George C., Wang, YuHuang·2013·Nature Chemistry

DOI 10.1038/nchem.1711

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Abstract

Semiconducting carbon nanotubes promise a broad range of potential applications in optoelectronics and imaging, but their photon-conversion efficiency is relatively low. Quantum theory suggests that nanotube photoluminescence is intrinsically inefficient because of low-lying 'dark' exciton states. Here we demonstrate the significant brightening of nanotube photoluminescence (up to 28-fold) through the creation of an optically allowed defect state that resides below the predicted energy level of the dark excitons. Emission from this new state generates a photoluminescence peak that is red-shifted by as much as 254 meV from the nanotube's original excitonic transition. We also found that the attachment of electron-withdrawing substituents to carbon nanotubes systematically drives this defect state further down the energy ladder. Our experiments show that the material's photoluminescence quantum yield increases exponentially as a function of the shifted emission energy. This work lays the foundation for chemical control of defect quantum states in low-dimensional carbon materials.

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Authors: Piao, Y., Meany, B., Powell, L. R., Valley, N., Kwon, H., Schatz, G. C., & Wang, Y.
Affiliations: University of Maryland, College Park (US)
Northwestern University (US)
Corresponding author: Wang, YuHuang
ORCID: Kwon, Hyejin
Schatz, George C.
Wang, YuHuang
Venue: Nature Chemistry
Publisher: Springer Science and Business Media LLC
Published: 2013-07-21
Volume: 5
Issue: 10
Pages: 840-845
ISSN: 1755-4330 (ISSN-L)
1755-4349
DOI: 10.1038/nchem.1711
OpenAlex: W2007554685
Cited by: 480
References: 34
Citations by year: 2026: 33 · 2025: 41 · 2024: 44 · 2023: 43 · 2022: 41 · 2021: 43 · 2020: 32 · 2019: 43 · 2018: 41 · 2017: 38 · 2016: 39 · 2015: 24 · 2014: 17 · 2013: 1
FWCI: 12.18
Type: journal article
Language: en
Open access: closed
Licence: www.springer.com/tdm (tdm)
Locations: Nature Chemistry (publishedVersion)
PubMed (publishedVersion)
Funders: Multidisciplinary University Research Initiative
Army Research Office
Topics: Physical Sciences › Materials Science › Materials Chemistry › Graphene research and applications
Physical Sciences › Materials Science › Materials Chemistry › Carbon Nanotubes in Composites
Physical Sciences › Materials Science › Materials Chemistry › Carbon and Quantum Dots Applications
Keywords: carbon nanotubes, sp3 defects, defect states, dark excitons, red-shifted emission, electron-withdrawing substituents, photoluminescence quantum yield, single-walled carbon nanotubes, chemical functionalization, photon conversion efficiency
MeSH terms: Electrons, Luminescent Measurements, Particle Size, Quantum Theory, Nanotubes, Carbon

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Brightening of carbon nanotube photoluminescence through the incorporation of sp3 defects

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