The DOI matches its Crossref record; 34 of the 34 references it cites were found in a registry or an index.
Wafer-sized multifunctional polyimine-based two-dimensional conjugated polymers with high mechanical stiffness
Open accessAbstract
One of the key challenges in two-dimensional (2D) materials is to go beyond graphene, a prototype 2D polymer (2DP), and to synthesize its organic analogues with structural control at the atomic- or molecular-level. Here we show the successful preparation of porphyrin-containing monolayer and multilayer 2DPs through Schiff-base polycondensation reaction at an air–water and liquid–liquid interface, respectively. Both the monolayer and multilayer 2DPs have crystalline structures as indicated by selected area electron diffraction. The monolayer 2DP has a thickness of∼0.7 nm with a lateral size of 4-inch wafer, and it has a Young’s modulus of 267±30 GPa. Notably, the monolayer 2DP functions as an active semiconducting layer in a thin film transistor, while the multilayer 2DP from cobalt-porphyrin monomer efficiently catalyses hydrogen generation from water. This work presents an advance in the synthesis of novel 2D materials for electronics and energy-related applications.
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Cited by
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Metadata
- Authors
- Sahabudeen, H., Qi, H., Glatz, B. A., Tranca, D., Dong, R., Hou, Y., Zhang, T., Kuttner, C., Lehnert, T., Seifert, G., Kaiser, U., Fery, A., Zheng, Z., & Feng, X.
- Venue
- Nature Communications
- Published
- 2016-11-16
- Volume
- 7
- Issue
- 1
- Pages
- 13461-13461
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2550509429
- Cited by
- 371
- References
- 34
- FWCI
- 15.13
- Type
- journal article
- Language
- en
- Open access
- gold
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- Sahabudeen, H., Qi, H., Glatz, B. A., Tranca, D., Dong, R., Hou, Y., Zhang, T., Kuttner, C., Lehnert, T., Seifert, G., Kaiser, U., Fery, A., Zheng, Z., & Feng, X. (2016). Wafer-sized multifunctional polyimine-based two-dimensional conjugated polymers with high mechanical stiffness. Nature Communications. https://doi.org/10.1038/ncomms13461
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