The DOI matches its Crossref record; 31 of the 31 references it cites were found in a registry or an index.
Self-assembled three-dimensional and compressible interdigitated thin-film supercapacitors and batteries
Open accessAbstract
Traditional thin-film energy-storage devices consist of stacked layers of active films on two-dimensional substrates and do not exploit the third dimension. Fully three-dimensional thin-film devices would allow energy storage in bulk materials with arbitrary form factors and with mechanical properties unique to bulk materials such as compressibility. Here we show three-dimensional energy-storage devices based on layer-by-layer self-assembly of interdigitated thin films on the surface of an open-cell aerogel substrate. We demonstrate a reversibly compressible three-dimensional supercapacitor with carbon nanotube electrodes and a three-dimensional hybrid battery with a copper hexacyanoferrate ion intercalating cathode and a carbon nanotube anode. The three-dimensional supercapacitor shows stable operation over 400 cycles with a capacitance of 25 F g−1 and is fully functional even at compressions up to 75%. Our results demonstrate that layer-by-layer self-assembly inside aerogels is a rapid, precise and scalable route for building high-surface-area 3D thin-film devices.
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Metadata
- Authors
- Nyström, G., Marais, A., Karabulut, E., Wågberg, L., Cui, Y., & Hamedi, M. M.
- Venue
- Nature Communications
- Published
- 2015-05-29
- Volume
- 6
- Issue
- 1
- Pages
- 7259-7259
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W946063174
- Cited by
- 280
- References
- 31
- FWCI
- 13.89
- Type
- journal article
- Language
- en
- Open access
- gold
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