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Cited by 773

The DOI matches its Crossref record; 32 of the 32 references it cites were found in a registry or an index.

Single-site trinuclear copper oxygen clusters in mordenite for selective conversion of methane to methanol

Open access
Grundner, Sebastian, Markovits, Monica A.C., Li, Guanna, Tromp, Moniek, Pidko, Evgeny A., Hensen, Emiel J.M., Jentys, Andreas, Sanchez-Sanchez, Maricruz, Lercher, Johannes A.·2015·Nature Communications
DOI 10.1038/ncomms8546
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Abstract

Copper-exchanged zeolites with mordenite structure mimic the nuclearity and reactivity of active sites in particulate methane monooxygenase, which are enzymes able to selectively oxidize methane to methanol. Here we show that the mordenite micropores provide a perfect confined environment for the highly selective stabilization of trinuclear copper-oxo clusters that exhibit a high reactivity towards activation of carbon–hydrogen bonds in methane and its subsequent transformation to methanol. The similarity with the enzymatic systems is also implied from the similarity of the reversible rearrangements of the trinuclear clusters occurring during the selective transformations of methane along the reaction path towards methanol, in both the enzyme system and copper-exchanged mordenite.

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Crossref · 10.1038/ncomms8546

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Metadata

Authors
Grundner, S., Markovits, M. A. C., Li, G., Tromp, M., Pidko, E. A., Hensen, E. J. M., Jentys, A., Sanchez-Sanchez, M., & Lercher, J. A.
Venue
Nature Communications
Publisher
Springer Science and Business Media LLC
Published
2015-06-25
Volume
6
Issue
1
Pages
7546-7546
ISSN
2041-1723 (ISSN-L)
DOI
10.1038/ncomms8546
OpenAlex
W2162783646
Cited by
773
References
32
FWCI
26.30
Type
journal article
Language
en
Open access
gold

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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.

Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).

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