Cited by 443Thermal properties of materialsThermoelastic and Magnetoelastic PhenomenaThermal Radiation and Cooling Technologies

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Quasi-ballistic thermal transport from nanoscale interfaces observed using ultrafast coherent soft X-ray beams

Siemens, Mark E., Li, Qing, Yang, Ronggui, Nelson, Keith A., Anderson, Erik H., Murnane, Margaret M., Kapteyn, Henry C.·2010·Nature Materials

DOI 10.1038/nmat2568

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Abstract

Fourier theory of thermal transport considers heat transport as a diffusive process where energy flow is driven by a temperature gradient. However, this is not valid at length scales smaller than the mean free path for the energy carriers in a material, which can be hundreds of nanometres in crystalline materials at room temperature. In this case, heat flow will become 'ballistic'--driven by direct point-to-point transport of energy quanta. Past experiments have demonstrated size-dependent ballistic thermal transport through nanostructures such as thin films, superlattices, nanowires and carbon nanotubes. The Fourier law should also break down in the case of heat dissipation from a nanoscale heat source into the bulk. However, despite considerable theoretical discussion and direct application to thermal management in nanoelectronics, nano-enabled energy systems and nanomedicine, this non-Fourier heat dissipation has not been experimentally observed so far. Here, we report the first observation and quantitative measurements of this transition from diffusive to ballistic thermal transport from a nanoscale hotspot, finding a significant (as much as three times) decrease in energy transport away from the nanoscale heat source compared with Fourier-law predictions.

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Authors: Siemens, M. E., Li, Q., Yang, R., Nelson, K. A., Anderson, E. H., Murnane, M. M., & Kapteyn, H. C.
Affiliations: Joint Institute for Laboratory Astrophysics (US)
University of Colorado Boulder (US)
Massachusetts Institute of Technology (US)
Lawrence Berkeley National Laboratory (US)
Corresponding author: Siemens, Mark E.
ORCID: Siemens, Mark E.
Li, Qing
Yang, Ronggui
Nelson, Keith A.
Anderson, Erik H.
Murnane, Margaret M.
Kapteyn, Henry C.
Venue: Nature Materials
Publisher: Springer Science and Business Media LLC
Published: 2009-11-08
Volume: 9
Issue: 1
Pages: 26-30
ISSN: 1476-1122 (ISSN-L)
1476-4660
DOI: 10.1038/nmat2568
OpenAlex: W2165930865
Cited by: 443
References: 29
Citations by year: 2026: 18 · 2025: 23 · 2024: 14 · 2023: 21 · 2022: 19 · 2021: 38 · 2020: 28 · 2019: 35 · 2018: 36 · 2017: 30 · 2016: 40 · 2015: 29 · 2014: 34 · 2013: 27 · 2012: 17
FWCI: 8.22
Type: journal article
Language: en
Open access: closed
Licence: www.springer.com/tdm (tdm)
www.springer.com/tdm (vor)
Locations: Nature Materials (publishedVersion)
PubMed (publishedVersion)
Funders: National Science Foundation
U.S. Department of Energy
Topics: Physical Sciences › Materials Science › Materials Chemistry › Thermal properties of materials
Physical Sciences › Engineering › Mechanics of Materials › Thermoelastic and Magnetoelastic Phenomena
Physical Sciences › Engineering › Civil and Structural Engineering › Thermal Radiation and Cooling Technologies
Keywords: ballistic thermal transport, nanoscale interfaces, non-Fourier heat conduction, nanoscale thermal management

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Quasi-ballistic thermal transport from nanoscale interfaces observed using ultrafast coherent soft X-ray beams

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