Domino-like multi-emissions across red and near infrared from solid-state 2-/2,6-aryl substituted BODIPY dyes
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Considerable achievements on multiple emission capabilities and tunable wavelengths have been obtained in inorganic luminescent materials. However, the development of organic counterparts remains a grand challenge. Herein we report a series of 2-/2,6-aryl substituted boron-dipyrromethene dyes with wide-range and multi-fluorescence emissions across red and near infrared in their aggregation states. Experimental data of X-ray diffraction, UV–vis absorption, and room temperature fluorescence spectra have proved the multiple excitation and easy-adjustable emission features in aggregated boron-dipyrromethene dyes. Temperature-dependent and time-resolved fluorescence studies have indicated a successive energy transfer from high to step-wisely lower-located energy levels that correspond to different excitation states of aggregates. Consistent quantum chemical calculation results have proposed possible aggregation modes of boron-dipyrromethene dyes to further support the above-described scenario. Thus, this study greatly enriches the fundamental recognition of conventional boron-dipyrromethene dyes by illustrating the relationships between multiple emission behaviors and the aggregation states of boron-dipyrromethene molecules.
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A spectral shift of the fluorescence emission was observed from 552 nm in THF to 605, 768, 868, and 976 nm in the multifluorescence microcrystalline states (formed at varied volumetric fractions of water and THF) with a decent Φfl (Φfl = 10%).
“A spectral shift of the fluorescence emission was observed from 552 nm in tetrahydrofuran (THF) to 605, 768, 868, and 976 nm in the multifluorescence microcrystalline states (formed at varied volumetric factions of water and THF) with a decent Φfl (Φfl = 10%).”
From The Pursuit of Shortwave Infrared-Emitting Nanoparticles with Bright Fluorescence through Molecular Design and Excited-State Engineering of Molecular Aggregates (2022) · cites this paper as [126]
Split into 2 atoms — 1 confirmed, 1 partially supported, 0 disputed, 0 misattributed, 0 unverifiable. Expand the claim to see per-atom verdicts.
Experimental — accuracy not yet measuredSuccessive domino-like energy transfer in 2-/2,6-aryl substituted BODIPY dyes (BDP1) has been observed from high to step-wisely lower-located energy levels corresponding to different excitation states of aggregates, which leads to multifluorescence emissions across red and NIR-SWIR in their aggregation states.
“Successive domino-like energy transfer in 2-/2,6-aryl substituted BODIPY dyes (BDP1) has been observed from high to step-wisely lower-located energy levels corresponding to different excitation states of aggregates, which leads to multifluorescence emissions across red and NIR-SWIR in their aggregation states (Figure 5b).126”
From The Pursuit of Shortwave Infrared-Emitting Nanoparticles with Bright Fluorescence through Molecular Design and Excited-State Engineering of Molecular Aggregates (2022) · cites this paper as [126]
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Self-citation
- Authors
- Tian, D., Qi, F., Ma, H., Wang, X., Pan, Y., Chen, R., Shen, Z., Liu, Z., Huang, L., & Huang, W.
- Affiliations
- Nanjing Tech University (CN)
- Nanjing University of Posts and Telecommunications (CN)
- Collaborative Innovation Center of Advanced Microstructures (CN)
- Corresponding author
- Shen, Zhen
- Liu, Zhipeng
- Huang, Ling
- ORCID
- Venue
- Nature Communications
- Published
- 2018-07-12
- Volume
- 9
- Issue
- 1
- Pages
- 2688-2688
- ISSN
- 2041-1723 (ISSN-L)
- PMC
- PMC6043560
- OpenAlex
- W2854672850
- Cited by
- 111
- References
- 42
- Citations by year
- 2026: 7 · 2025: 8 · 2024: 13 · 2023: 17 · 2022: 14 · 2021: 17 · 2020: 18 · 2019: 16 · 2018: 1
- FWCI
- 4.85
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Locations
- Nature Communications (publishedVersion, cc-by)
- Europe PMC (PubMed Central) (publishedVersion, other-oa)
- PubMed Central (publishedVersion, cc-by)
- PubMed (publishedVersion)
- RePEc: Research Papers in Economics (submittedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- Funders
- National Natural Science Foundation of China (21371095)
- Topics
- Physical Sciences › Materials Science › Materials Chemistry › Luminescence and Fluorescent Materials
- Physical Sciences › Chemistry › Spectroscopy › Molecular Sensors and Ion Detection
- Physical Sciences › Chemistry › Physical and Theoretical Chemistry › Photochemistry and Electron Transfer Studies
- Keywords
- BODIPY dyes, boron dipyrromethene, red fluorescence, near-infrared emission, aggregation-induced emission, aggregation state, excitation states, quantum chemical calculations, aggregation modes
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