The DOI matches its Crossref record; 37 of the 37 references it cites were found in a registry or an index.
High capacity silicon anodes enabled by MXene viscous aqueous ink
Open accessAbstract
The ever-increasing demands for advanced lithium-ion batteries have greatly stimulated the quest for robust electrodes with a high areal capacity. Producing thick electrodes from a high-performance active material would maximize this parameter. However, above a critical thickness, solution-processed films typically encounter electrical/mechanical problems, limiting the achievable areal capacity and rate performance as a result. Herein, we show that two-dimensional titanium carbide or carbonitride nanosheets, known as MXenes, can be used as a conductive binder for silicon electrodes produced by a simple and scalable slurry-casting technique without the need of any other additives. The nanosheets form a continuous metallic network, enable fast charge transport and provide good mechanical reinforcement for the thick electrode (up to 450 µm). Consequently, very high areal capacity anodes (up to 23.3 mAh cm−2) have been demonstrated.
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Cites
Two‐Dimensional Nanocrystals Produced by Exfoliation of Ti3AlC2
Naguib, M., Kurtoglu, M., Presser, V., Lu, J., Niu, J., Heon, M., Hultman, L., Gogotsi, Y., & Barsoum, M. W. (2011) · Advanced Materials · doi:10.1002/adma.201102306 · Cited by 11,855
Self-citationNano-sized transition-metal oxides as negative-electrode materials for lithium-ion batteries
Poizot, P., Laruelle, S., Grugeon, S., Dupont, L., & Tarascon, J.-M. (2000) · Nature · doi:10.1038/35035045 · Cited by 8,041
2D metal carbides and nitrides (MXenes) for energy storage
Anasori, B., Lukatskaya, M. R., & Gogotsi, Y. (2017) · Nature Reviews Materials · doi:10.1038/natrevmats.2016.98 · Cited by 7,440
Self-citationLi-ion battery materials: present and future
Nitta, N., Wu, F., Lee, J. T., & Yushin, G. (2015) · Materials Today · doi:10.1016/j.mattod.2014.10.040 · Cited by 7,389
Guidelines for Synthesis and Processing of Two-Dimensional Titanium Carbide (Ti3C2Tx MXene)
Alhabeb, M., Maleski, K., Anasori, B., Lelyukh, P., Clark, L., Sin, S., & Gogotsi, Y. (2017) · Chemistry of Materials · doi:10.1021/acs.chemmater.7b02847 · Cited by 5,045
Self-citationTwo-Dimensional Transition Metal Carbides
Naguib, M., Mashtalir, O., Carle, J., Presser, V., Lu, J., Hultman, L., Gogotsi, Y., & Barsoum, M. W. (2012) · ACS Nano · doi:10.1021/nn204153h · Cited by 4,769
Self-citationPaton, K. R., Varrla, E., Backes, C., Smith, R. J., Khan, U., O’Neill, A., Boland, C., Lotya, M., Istrate, O. M., King, P., et al. (2014) · Nature Materials · doi:10.1038/nmat3944 · Cited by 2,401
Self-citationTwo-Dimensional, Ordered, Double Transition Metals Carbides (MXenes)
Anasori, B., Xie, Y., Beidaghi, M., Lu, J., Hosler, B. C., Hultman, L., Kent, P. R. C., Gogotsi, Y., & Barsoum, M. W. (2015) · ACS Nano · doi:10.1021/acsnano.5b03591 · Cited by 2,110
Self-citationLipatov, A., Alhabeb, M., Lukatskaya, M. R., Boson, A., Gogotsi, Y., & Sinitskii, A. (2016) · Advanced Electronic Materials · doi:10.1002/aelm.201600255 · Cited by 1,751
Self-citationOxidation Stability of Colloidal Two-Dimensional Titanium Carbides (MXenes)
Zhang, C. J., Pinilla, S., McEvoy, N., Cullen, C. P., Anasori, B., Long, E., Park, S.-H., Seral-Ascaso, A., Shmeliov, A., Krishnan, D., et al. (2017) · Chemistry of Materials · doi:10.1021/acs.chemmater.7b00745 · Cited by 1,725
Self-citation
Cited by
Ten Years of Progress in the Synthesis and Development of MXenes
Naguib, M., Barsoum, M. W., & Gogotsi, Y. (2021) · Advanced Materials · doi:10.1002/adma.202103393 · Cited by 1,257
Self-citationHui, X., Zhao, R., Zhang, P., Li, C., Wang, C., & Yin, L. (2019) · Advanced Energy Materials · doi:10.1002/aenm.201901065 · Cited by 365
Hao, S., Han, H., Yang, Z., Chen, M., Jiang, Y., Lu, G., Dong, L., Wen, H., Li, H., Liu, J., et al. (2022) · Nano-Micro Letters · doi:10.1007/s40820-022-00901-w · Cited by 280
Metadata
- Authors
- Zhang, C., Park, S.-H., Seral‐Ascaso, A., Barwich, S., McEvoy, N., Boland, C. S., Coleman, J. N., Gogotsi, Y., & Nicolosi, V.
- Venue
- Nature Communications
- Published
- 2019-02-20
- Volume
- 10
- Issue
- 1
- Pages
- 849-849
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2916564885
- Cited by
- 365
- References
- 37
- FWCI
- 18.77
- Type
- journal article
- Language
- en
- Open access
- gold
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