The DOI matches its Crossref record; 18 of the 18 references it cites were found in a registry or an index.
Electrochemical CO2 reduction to high-concentration pure formic acid solutions in an all-solid-state reactor
Open accessAbstract
Electrochemical CO 2 reduction reaction (CO 2 RR) to liquid fuels is currently challenged by low product concentrations, as well as their mixture with traditional liquid electrolytes, such as KHCO 3 solution. Here we report an all-solid-state electrochemical CO 2 RR system for continuous generation of high-purity and high-concentration formic acid vapors and solutions. The cathode and anode were separated by a porous solid electrolyte (PSE) layer, where electrochemically generated formate and proton were recombined to form molecular formic acid. The generated formic acid can be efficiently removed in the form of vapors via inert gas stream flowing through the PSE layer. Coupling with a high activity (formate partial current densities ~450 mA cm−2), selectivity (maximal Faradaic efficiency ~97%), and stability (100 hours) grain boundary-enriched bismuth catalyst, we demonstrated ultra-high concentrations of pure formic acid solutions (up to nearly 100 wt.%) condensed from generated vapors via flexible tuning of the carrier gas stream.
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Metadata
- Authors
- Fan, L., Xia, C., Zhu, P., Lu, Y., & Wang, H.
- Venue
- Nature Communications
- Published
- 2020-07-20
- Volume
- 11
- Issue
- 1
- Pages
- 3633-3633
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3042815916
- Cited by
- 583
- References
- 18
- FWCI
- 13.15
- Type
- journal article
- Language
- en
- Open access
- gold
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- Fan, L., Xia, C., Zhu, P., Lu, Y., & Wang, H. (2020). Electrochemical CO2 reduction to high-concentration pure formic acid solutions in an all-solid-state reactor. Nature Communications. https://doi.org/10.1038/s41467-020-17403-1
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