The DOI matches its Crossref record; 7 of the 7 references it cites were found in a registry or an index.
Interface chemistry of an amide electrolyte for highly reversible lithium metal batteries
Open accessAbstract
Metallic lithium is a promising anode to increase the energy density of rechargeable lithium batteries. Despite extensive efforts, detrimental reactivity of lithium metal with electrolytes and uncontrolled dendrite growth remain challenging interconnected issues hindering highly reversible Li-metal batteries. Herein, we report a rationally designed amide-based electrolyte based on the desired interface products. This amide electrolyte achieves a high average Coulombic efficiency during cycling, resulting in an outstanding capacity retention with a 3.5 mAh cm−2 high-mass-loaded LiNi 0.8 Co 0.1 Mn 0.1 O 2 cathode. The interface reactions with the amide electrolyte lead to the predicted solid electrolyte interface species, having favorable properties such as high ionic conductivity and high stability. Operando monitoring the lithium spatial distribution reveals that the highly reversible behavior is related to denser deposition as well as top-down stripping, which decreases the formation of porous deposits and inactive lithium, providing new insights for the development of interface chemistries for metal batteries.
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Fluoroethylene Carbonate Additives to Render Uniform Li Deposits in Lithium Metal Batteries
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Atomic structure of sensitive battery materials and interfaces revealed by cryo–electron microscopy
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High-Efficiency Lithium Metal Batteries with Fire-Retardant Electrolytes
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Perspective—Fluorinating Interphases
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Cited by
Li, Z., Yu, R., Weng, S., Zhang, Q., Wang, X., & Guo, X. (2023) · Nature Communications · doi:10.1038/s41467-023-35857-x · Cited by 341
Wu, D., He, J., Liu, J., Wu, M., Qi, S., Wang, H., Huang, J., Li, F., Tang, D., & Ma, J. (2022) · Advanced Energy Materials · doi:10.1002/aenm.202200337 · Cited by 319
High entropy liquid electrolytes for lithium batteries
Wang, Q., Zhao, C., Wang, J., Yao, Z., Wang, S., Kumar, S. G. H., Ganapathy, S., Eustace, S., Bai, X., Li, B., et al. (2023) · Nature Communications · doi:10.1038/s41467-023-36075-1 · Cited by 299
Self-citationWu, Z., Li, R., Zhang, S., lv, L., Deng, T., Zhang, H., Zhang, R., Liu, J., Ding, S., Fan, L., et al. (2023) · Chem · doi:10.1016/j.chempr.2022.10.027 · Cited by 282
Insights into the deposition chemistry of Li ions in nonaqueous electrolyte for stable Li anodes
Wang, Z., Sun, Z., Li, J., Shi, Y., Sun, C., An, B., Cheng, H.-M., & Li, F. (2021) · Chemical Society Reviews · doi:10.1039/d0cs01017k · Cited by 268
Metadata
- Authors
- Wang, Q., Yao, Z., Zhao, C., Verhallen, T., Tabor, D. P., Liu, M., Ooms, F., Kang, F., Aspuru-Guzik, A., Hu, Y.-S., Wagemaker, M., & Li, B.
- Venue
- Nature Communications
- Published
- 2020-08-21
- Volume
- 11
- Issue
- 1
- Pages
- 4188-4188
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3080822653
- Cited by
- 427
- References
- 7
- FWCI
- 18.31
- Type
- journal article
- Language
- en
- Open access
- gold
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- Wang, Q., Yao, Z., Zhao, C., Verhallen, T., Tabor, D. P., Liu, M., Ooms, F., Kang, F., Aspuru-Guzik, A., Hu, Y.-S., Wagemaker, M., & Li, B. (2020). Interface chemistry of an amide electrolyte for highly reversible lithium metal batteries. Nature Communications. https://doi.org/10.1038/s41467-020-17976-x
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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