The DOI matches its Crossref record; 9 of the 9 references it cites were found in a registry or an index.
Engineering active sites on hierarchical transition bimetal oxides/sulfides heterostructure array enabling robust overall water splitting
Open accessAbstract
Rational design of the catalysts is impressive for sustainable energy conversion. However, there is a grand challenge to engineer active sites at the interface. Herein, hierarchical transition bimetal oxides/sulfides heterostructure arrays interacting two-dimensional MoO x/MoS 2 nanosheets attached to one-dimensional NiO x/Ni 3 S 2 nanorods were fabricated by oxidation/hydrogenation-induced surface reconfiguration strategy. The NiMoO x/NiMoS heterostructure array exhibits the overpotentials of 38 mV for hydrogen evolution and 186 mV for oxygen evolution at 10 mA cm−2, even surviving at a large current density of 500 mA cm−2 with long-term stability. Due to optimized adsorption energies and accelerated water splitting kinetics by theory calculations, the assembled two-electrode cell delivers the industrially relevant current densities of 500 and 1000 mA cm−2 at record low cell voltages of 1.60 and 1.66 V with excellent durability. This research provides a promising avenue to enhance the electrocatalytic performance of the catalysts by engineering interfacial active sites toward large-scale water splitting.
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Cites
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Cited by
Chen, J., Long, Q., Xiao, K., Ouyang, T., Li, N., Ye, S., & Liu, Z.-Q. (2021) · Science Bulletin · doi:10.1016/j.scib.2021.02.033 · Cited by 363
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Engineering β-ketoamine covalent organic frameworks for photocatalytic overall water splitting
Yang, Y., Chu, X., Zhang, H.-Y., Zhang, R., Liu, Y.-H., Zhang, F.-M., Lu, M., Yang, Z.-D., & Lan, Y.-Q. (2023) · Nature Communications · doi:10.1038/s41467-023-36338-x · Cited by 281
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Progress and Perspectives for Solar‐Driven Water Electrolysis to Produce Green Hydrogen
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Metadata
- Authors
- Zhai, P., Zhang, Y., Wu, Y., Gao, J., Zhang, B., Cao, S., Zhang, Y., Li, Z., Sun, L., & Hou, J.
- Venue
- Nature Communications
- Published
- 2020-10-29
- Volume
- 11
- Issue
- 1
- Pages
- 5462-5462
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3095015225
- Cited by
- 673
- References
- 9
- FWCI
- 17.54
- Type
- journal article
- Language
- en
- Open access
- gold
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- Zhai, P., Zhang, Y., Wu, Y., Gao, J., Zhang, B., Cao, S., Zhang, Y., Li, Z., Sun, L., & Hou, J. (2020). Engineering active sites on hierarchical transition bimetal oxides/sulfides heterostructure array enabling robust overall water splitting. Nature Communications. https://doi.org/10.1038/s41467-020-19214-w
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