Fire-extinguishing, recyclable liquefied gas electrolytes for temperature-resilient lithium-metal batteries
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In rationally designed LGEs, solvated FSI- and dimethyl ether dominate the solvation structure, which is believed to reduce the free Me2O solvent amount, leading to improved oxidative stability and salt decomposition to form a LiF-rich SEI on the anode.
“In rationally designed LGEs, solvated FSI -and dimethyl ether (Me 2 O) dominate the solvation structure, which is believed to reduce the free Me 2 O solvent amount leading to the improvement of the oxidative stability and the salt decomposition to form a LiF-rich SEI on the anode.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [78]
Meng's group developed a novel LGE by adding the simplest liquefied ether to a non-flammable low-solvating hydrofluorocarbon mixture.
“Meng's group [78] recently developed a novel LGE by adding the simplest (liquefied) ether to a non-flammable lowsolvating hydrofluorocarbon mixture.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [78]
The LGE with oxidation stability up to 4.4 V enabled Li/NMC622 cells to exhibit stable cycling properties from -60 to 55 °C.
“The LGE with oxidation stability up to 4.4 V enabled Li/NMC622 cells exhibiting stable cycling properties from -60 to 55 °C.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [78]
The LGE based on 1,1,1,2-tetrafluoroethane and pentafluoroethane delivered high ionic conductivity >3 mS cm-1 from -78 to 80 °C, with non-flammable and fire-extinguishing features.
“The LGE based on 1,1,1,2-tetrafluoroethane and pentafluoroethane delivered high ionic conductivity > 3 mS cm -1 within the temperature range from -78 to 80 °C, with non-flammable and fireextinguishing features.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [78]
Lithium cycling at >99% Coulombic efficiency for over 200 cycles at 3 mA cm-2 and 3 mAh cm-2 was demonstrated.
“As a result of the beneficial solvation chemistry and a fluorine-rich environment, a lithium cycling at > 99% Coulombic efficiency for over 200 cycles at 3 mA cm -2 and 3 mAh cm -2 was demonstrated.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [78]
Within the wide temperature range, LMBs retained Coulombic efficiencies of 97.3%, 97.2%, 95.2%, and 91.0% at 0, -20, -40, and -60 °C, respectively.
“Moreover, within the widetemperature range, LMBs retained Coulombic efficiencies of 97.3%, 97.2%, 95.2% and 91.0% at 0, -20, -40 and -60 °C, respectively.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [78]
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Challenges and Advances in Wide‐Temperature Electrolytes for Lithium‐Ion Batteries
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“71 The charge/discharge process during battery cycling is driven by the movement of solvated Li þ ions in the electrolyte and their reaction at the anode.”
Liquid Metal-Skinned Zn Powder Anodes Enabled by Capillary Suspension
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Macromolecular Boron‐Based Salt Enables Dense Interphases for Long‐Cycling Lithium‐Sulfur Batteries
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“In addition, current commercialized electrolytes exhibit a narrow operational temperature window (0° to 45°C) ( 8 ), rendering them unsuitable for extreme temperature applications ( 9 , 10 ).”
Linear ether-based highly concentrated electrolytes for Li–sulfur batteries
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Correlating Solvation Free Energy to Electrolyte Properties for Lithium Metal Batteries.
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Electrolytic construction of nanosphere‐assembled protective layer toward stable lithium metal anode
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- Authors
- Yin, Y., Yang, Y., Cheng, D., Mayer, M., Holoubek, J., Li, W., Raghavendran, G., Liu, A., Lu, B., Davies, D. M., Chen, Z., Borodin, O., & Meng, Y. S.
- Affiliations
- University of California San Diego (US)
- DEVCOM Army Research Laboratory (US)
- Corresponding author
- Yang, Yangyuchen
- Borodin, Oleg
- Meng, Y. Shirley
- ORCID
- Venue
- Nature Energy
- Published
- 2022-06-16
- Volume
- 7
- Issue
- 6
- Pages
- 548-559
- ISSN
- 2058-7546 (ISSN-L)
- OpenAlex
- W4283027379
- Cited by
- 150
- References
- 52
- Citations by year
- 2026: 19 · 2025: 39 · 2024: 41 · 2023: 42 · 2022: 9
- FWCI
- 8.97
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Nature Energy (publishedVersion)
- RePEc: Research Papers in Economics (submittedVersion)
- Funders
- Sustainable Power and Energy Center and Zable endowed chair fund for energy technologies
- DOE | Office of Energy Efficiency & Renewable Energy | Vehicle Technologies Office (DE-SC0012704)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
- Physical Sciences › Engineering › Automotive Engineering › Advanced Battery Technologies Research
- Keywords
- lithium metal batteries, R134a, pentafluoroethane, temperature resilience, ionic conductivity, Coulombic efficiency, solvent recovery, fluorinated solvents, battery safety
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