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A Highly Reversible Lithium Metal Anode
Open accessAbstract
Lithium metal has shown a lot of promise for use as an anode material in rechargeable batteries owing to its high theoretical capacity. However, it does not meet the cycle life and safety requirements of rechargeable batteries owing to electrolyte decomposition and dendrite formation on the surfaces of the lithium anodes during electrochemical cycling. Here, we propose a novel electrolyte system that is relatively stable against lithium metal and mitigates dendritic growth. Systematic design methods that combined simulations, model-based experiments, and in situ analyses were employed to design the system. The reduction potential of the solvent, the size of the salt anions, and the viscosity of the electrolyte were found to be critical parameters determining the rate of dendritic growth. A lithium metal anode in contact with the designed electrolyte exhibited remarkable cyclability (more than 100 cycles) at a high areal capacity of 12 mAh cm(-2).
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Cites
Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Cited by
High rate and stable cycling of lithium metal anode
Qian, J., Henderson, W. A., Xu, W., Bhattacharya, P., Engelhard, M., Borodin, O., & Zhang, J.-G. (2015) · Nature Communications · doi:10.1038/ncomms7362 · Cited by 2,561
The synergetic effect of lithium polysulfide and lithium nitrate to prevent lithium dendrite growth
Li, W., Yao, H., Yan, K., Zheng, G., Liang, Z., Chiang, Y.-M., & Cui, Y. (2015) · Nature Communications · doi:10.1038/ncomms8436 · Cited by 1,540
Sodium Metal Anodes: Emerging Solutions to Dendrite Growth
Lee, B., Paek, E., Mitlin, D., & Lee, S. W. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00642 · Cited by 940
Li plating as unwanted side reaction in commercial Li-ion cells – A review
Waldmann, T., Hogg, B.-I., & Wohlfahrt-Mehrens, M. (2018) · Journal of Power Sources · doi:10.1016/j.jpowsour.2018.02.063 · Cited by 895
3D Porous Cu Current Collector/Li‐Metal Composite Anode for Stable Lithium‐Metal Batteries
Li, Q., Zhu, S., & Lu, Y. (2017) · Advanced Functional Materials · doi:10.1002/adfm.201606422 · Cited by 854
Metadata
- Authors
- Park, M. S., Ma, S. B., Lee, D. J., Im, D., Doo, S.-G., & Yamamoto, O.
- Venue
- Scientific Reports
- Published
- 2014-01-22
- Volume
- 4
- Issue
- 1
- Pages
- 3815-3815
- ISSN
- 2045-2322 (ISSN-L)
- OpenAlex
- W1982339678
- Cited by
- 339
- References
- 1
- FWCI
- 17.69
- Type
- journal article
- Language
- en
- Open access
- gold
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- Park, M. S., Ma, S. B., Lee, D. J., Im, D., Doo, S.-G., & Yamamoto, O. (2014). A Highly Reversible Lithium Metal Anode. Scientific Reports. https://doi.org/10.1038/srep03815
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
