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A hierarchical view on material formation during pulsed-laser synthesis of nanoparticles in liquid

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Ibrahimkutty, Shyjumon, Wagener, Philipp, Rolo, Tomy dos Santos, Karpov, Dmitry, Menzel, Andreas, Baumbach, Tilo, Barcikowski, Stephan, Plech, Anton·2015·Scientific Reports
DOI 10.1038/srep16313
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Abstract

Pulsed-laser assisted nanoparticle synthesis in liquids (PLAL) is a versatile tool for nanoparticle synthesis. However, fundamental aspects of structure formation during PLAL are presently poorly understood. We analyse the spatio-temporal kinetics during PLAL by means of fast X-ray radiography (XR) and scanning small-angle X-ray scattering (SAXS), which permits us to probe the process on length scales from nanometers to millimeters with microsecond temporal resolution. We find that the global structural evolution, such as the dynamics of the vapor bubble can be correlated to the locus and evolution of silver nanoparticles. The bubble plays an important role in particle formation, as it confines the primary particles and redeposits them to the substrate. Agglomeration takes place for the confined particles in the second bubble. Additionally, upon the collapse of the second bubble a jet of confined material is ejected perpendicularly to the surface. We hypothesize that these kinetics influence the final particle size distribution and determine the quality of the resulting colloids, such as polydispersity and modality through the interplay between particle cloud compression and particle release into the liquid.

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Metadata

Authors
Ibrahimkutty, S., Wagener, P., Rolo, T. D. S., Karpov, D., Menzel, A., Baumbach, T., Barcikowski, S., & Plech, A.
Venue
Scientific Reports
Publisher
Springer Science and Business Media LLC
Published
2015-11-09
Volume
5
Issue
1
Pages
16313-16313
ISSN
2045-2322 (ISSN-L)
DOI
10.1038/srep16313
OpenAlex
W2192977715
Cited by
171
References
13
FWCI
10.54
Type
journal article
Language
en
Open access
gold
Licence

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CoChat. (2026). Citation check: A hierarchical view on material formation during pulsed-laser synthesis of nanoparticles in liquid. https://app.cochat.ai/papers/10.1038/srep16313
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Ibrahimkutty, S., Wagener, P., Rolo, T. D. S., Karpov, D., Menzel, A., Baumbach, T., Barcikowski, S., & Plech, A. (2015). A hierarchical view on material formation during pulsed-laser synthesis of nanoparticles in liquid. Scientific Reports. https://doi.org/10.1038/srep16313

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