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Cited by 92Molecular spectroscopy and chiralityMolecular Spectroscopy and StructureAdvanced Chemical Physics Studies

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Recent experimental and theoretical developments towards the observation of parity violation (PV) effects in molecules by spectroscopy

Crassous, Jeanne, Chardonnet, Christian, Saue, Trond, Schwerdtfeger, Peter·2005·Organic & Biomolecular Chemistry
DOI 10.1039/b504212g
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Abstract

Parity violation (PV) at the molecular level is known to be responsible for a tiny energy difference between the two enantiomers of a chiral molecule. This parity violation energy difference (PVED) has not yet been detected by experiment. In the last few years, the search for PV effects in molecules has made important steps ahead for several reasons. On one hand, very accurate infra-red spectroscopy measurements were performed by metrologists on bromochlorofluoromethane (CHFClBr) with a 10 Hz accuracy, which so far is the most precise. On the other hand, relativistic calculations were used for the evaluation of DeltaE(PV) allowing for a screening of favorable molecules for future measurements. The synthesis of such chiral molecules with high parity violation effects is currently being investigated. In memory of Professor Jean-Bernard Robert.

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  • No observation has unambiguously confirmed parity violation energy difference in chiral molecules yet.

    “Although groups of Crassous/ Darquie ´in France 78,[93][94][95][96][97][98] and Quack in Switzerland [99][100][101][102][103] have been pursuing an experimental effort to measure PVED, thanks to approaches based on spectroscopic techniques and/or tunneling processes, no observation has unambiguously confirmed it yet.”

    From Possible chemical and physical scenarios towards biological homochirality (2022) · cites this paper as [78]

  • A parity violation energy difference of about 10^-17 kT at 300 K should be measurable by any absorption spectroscopy provided that ultra-high resolution can be reached.

    “Such a tiny parity violation energy difference (a PVED of about 10 À17 kT at 300 K) should be measurable by any absorption spectroscopy provided that ultra-high resolution can be reached.[78][79][80][81]”

    From Possible chemical and physical scenarios towards biological homochirality (2022) · cites this paper as [78]

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Metadata

Authors
Crassous, J., Chardonnet, C., Saue, T., & Schwerdtfeger, P.
Affiliations
  • École Normale Supérieure de Lyon (FR)
  • Centre National de la Recherche Scientifique (FR)
  • Massey University (NZ)
Corresponding author
Crassous, Jeanne
ORCID
Venue
Organic & Biomolecular Chemistry
Publisher
Royal Society of Chemistry (RSC)
Published
2005
Volume
3
Issue
12
Pages
2218
ISSN
  • 1477-0520 (ISSN-L)
  • 1477-0539
DOI
10.1039/b504212g
OpenAlex
W1980875638
Cited by
92
References
2
Citations by year
2026: 2 · 2025: 1 · 2024: 2 · 2023: 2 · 2022: 3 · 2021: 2 · 2020: 2 · 2019: 2 · 2018: 2 · 2017: 2 · 2014: 3 · 2013: 4 · 2012: 7
FWCI
3.49
Type
journal article
Language
en
Open access
closed
Locations
  • Organic & Biomolecular Chemistry (publishedVersion)
  • PubMed (publishedVersion)
Topics
  • Physical Sciences › Chemistry › Spectroscopy › Molecular spectroscopy and chirality
  • Physical Sciences › Chemistry › Spectroscopy › Molecular Spectroscopy and Structure
  • Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Advanced Chemical Physics Studies
Keywords
parity violation, chiral molecules, enantiomers, infrared spectroscopy, relativistic calculations, molecular chirality

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