The DOI matches its Crossref record; 144 of the 144 references it cites were found in a registry or an index.
Catalysis for CO2 conversion: a key technology for rapid introduction of renewable energy in the value chain of chemical industries
Abstract
Replacement of part of the fossil fuel consumption by renewable energy, in particular in the chemical industry, is a central strategy for resource and energy efficiency. This perspective will show that CO2 is the key molecule to proceed effectively in this direction. The routes, opportunities and barriers in increasing the share of renewable energy by using CO2 reaction and their impact on the chemical and energy value chains are discussed after introducing the general aspects of this topic evidencing the tight integration between the CO2 use and renewable energy insertion in the value chain of the process industry. The focus of this perspective article is on the catalytic aspects of the chemistries involved, with an analysis of the state-of-the-art, perspectives and targets to be developed. The reactions discussed are the production of short-chain olefins (ethylene, propylene) from CO2, and the conversion of carbon dioxide to syngas, formic acid, methanol and dimethyl ether, hydrocarbons via Fischer–Tropsch synthesis and methane. The relevance of availability, cost and environmental footprints of H2 production routes using renewable energies is addressed. The final part discusses the possible scenario for CO2 as an intermediary for the incorporation of renewable energy in the process industry, with a concise roadmap for catalysis needs and barriers to reach this goal.
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Cites
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Cited by
Carbon capture and storage (CCS): the way forward
Bui, M., Adjiman, C. S., Bardow, A., Anthony, E. J., Boston, A., Brown, S., Fennell, P. S., Fuss, S., Galindo, A., Hackett, L. A., et al. (2018) · Energy & Environmental Science · doi:10.1039/c7ee02342a · Cited by 4,374
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Klankermayer, J., Wesselbaum, S., Beydoun, K., & Leitner, W. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201507458 · Cited by 856
Metal‐Free Carbon Materials for CO2 Electrochemical Reduction
Duan, X., Xu, J., Wei, Z., Ma, J., Guo, S., Wang, S., Liu, H., & Dou, S. (2017) · Advanced Materials · doi:10.1002/adma.201701784 · Cited by 754
Climate change mitigation potential of carbon capture and utilization in the chemical industry
Kätelhön, A., Meys, R., Deutz, S., Suh, S., & Bardow, A. (2019) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1821029116 · Cited by 643
Metadata
- Authors
- Centi, G., Quadrelli, E. A., & Perathoner, S.
- Venue
- Energy & Environmental Science
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2013
- Volume
- 6
- Issue
- 6
- Pages
- 1711
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W2154304209
- Cited by
- 1,257
- References
- 144
- FWCI
- 33.91
- Type
- journal article
- Language
- en
- Open access
- closed
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- Centi, G., Quadrelli, E. A., & Perathoner, S. (2013). Catalysis for CO2 conversion: a key technology for rapid introduction of renewable energy in the value chain of chemical industries. Energy & Environmental Science. https://doi.org/10.1039/c3ee00056g
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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