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Au@TiO2yolk–shell hollow spheres for plasmon-induced photocatalytic reduction of CO2to solar fuel via a local electromagnetic field
Abstract
An electric field in a photocatalytic system consisting of Au@TiO2 yolk-shell hollow spheres is created to enhance the generation of electron-hole pairs and remit the charge-carrier recombination. Local surface plasmon resonance (LSPR)-mediated local electromagnetic field nearby Au nanoparticles cannot only enhance the local generation and subsequent separation of electron-hole pairs in TiO2 shells to improve the photoreduction yield of CO2, but also facilitate chemical reactions involving multiple e(-)/H(+) transfer processes to allow the formation of high-grade carbon species (C2H6), which was rarely observed in precedent CO2 photocatalytic reduction systems. The work may provide a new viewpoint for designing photocatalysts for artificial photosynthesis involving multiple reactions.
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Cited by
Recent Advances in Heterogeneous Photocatalytic CO 2 Conversion to Solar Fuels
Li, K., Peng, B., & Peng, T. (2016) · ACS Catalysis · doi:10.1021/acscatal.6b02089 · Cited by 1,355
Plasmon-Enhanced Photocatalytic CO2 Conversion within Metal–Organic Frameworks under Visible Light
Choi, K. M., Kim, D., Rungtaweevoranit, B., Trickett, C. A., Barmanbek, J. T. D., Alshammari, A. S., Yang, P., & Yaghi, O. M. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.6b11027 · Cited by 632
Kovačič, Ž., Likozar, B., & Huš, M. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c02557 · Cited by 474
Vu, N., Kaliaguine, S., & Do, T. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201901825 · Cited by 445
Metadata
- Authors
- Tu, W., Zhou, Y., Li, H., Li, P., & Zou, Z.
- Venue
- Nanoscale
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2015
- Volume
- 7
- Issue
- 34
- Pages
- 14232-14236
- ISSN
- 2040-3364 (ISSN-L)
- 2040-3372
- OpenAlex
- W1878070950
- Cited by
- 174
- References
- 0
- FWCI
- 6.16
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Au@TiO2yolk–shell hollow spheres for plasmon-induced photocatalytic reduction of CO2to solar fuel via a local electromagnetic field. https://app.cochat.ai/papers/10.1039/c5nr02943k
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- Tu, W., Zhou, Y., Li, H., Li, P., & Zou, Z. (2015). Au@TiO2yolk–shell hollow spheres for plasmon-induced photocatalytic reduction of CO2to solar fuel via a local electromagnetic field. Nanoscale. https://doi.org/10.1039/c5nr02943k
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