Nitrogen-doped graphenes as efficient electrocatalysts for the selective reduction of carbon dioxide to formate in aqueous solution
Abstract
We report the first example of metal-free nitrogen-doped graphene-based materials for the electrochemical reduction of CO 2 to formate. The synthesized catalysts are highly active and stable in the electrocatalytic reduction of CO 2 to formate in an aqueous electrolyte.
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The higher ID/IG ratio (1.18) for both CoFeO@N/S-rGO and CoFe@N-rGO compared to GO (0.88) indicates increased surface defects due to heteroatom doping and the deposition of nanoparticles.
“In comparison with GO (0.88), the higher ID/IG ratio (1.18) for both CoFeO@N/S-rGO and CoFe@N-rGO indicates increased surface defects due to heteroatom doping and the deposition of nanoparticles.30”
From Tunable CoFe-based active sites on 3D heteroatom doped graphene aerogel electrocatalysts <i>via</i> annealing gas regulation for efficient water splitting (2018) · cites this paper as [30]
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- Authors
- Wang, H., Chen, Y., Hou, X., Ma, C., & Tan, T.
- Affiliations
- Beijing University of Chemical Technology (CN)
- University of California System (US)
- Corresponding author
- Tan, Tianwei
- Venue
- Green Chemistry
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2016
- Volume
- 18
- Issue
- 11
- Pages
- 3250-3256
- ISSN
- 1463-9262 (ISSN-L)
- 1463-9270
- OpenAlex
- W2328258692
- Cited by
- 288
- References
- 0
- Citations by year
- 2026: 8 · 2025: 11 · 2024: 30 · 2023: 23 · 2022: 31 · 2021: 29 · 2020: 42 · 2019: 44 · 2018: 36 · 2017: 27 · 2016: 7
- FWCI
- 10.32
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Green Chemistry (publishedVersion)
- Funders
- National Natural Science Foundation of China
- National Key Research and Development Program of China
- Division of Materials Research
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Chemical Engineering › Process Chemistry and Technology › Carbon dioxide utilization in catalysis
- Keywords
- nitrogen-doped graphene, electrocatalysis, CO2 reduction, formate production, metal-free catalysts, aqueous electrolyte solutions, electrocatalyst stability
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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